Department of Physics, University of Oxford, Clarendon Laboratory, Oxford, OX1 3PU, United Kingdom.
Phys Rev Lett. 2012 Dec 7;109(23):237202. doi: 10.1103/PhysRevLett.109.237202. Epub 2012 Dec 3.
We have measured the spin-wave spectrum of the half-doped bilayer manganite Pr(Ca,Sr)(2)Mn(2)O(7) in its spin, charge, and orbital ordered phase. The measurements, which extend throughout the Brillouin zone and cover the entire one-magnon spectrum, are compared critically with spin-wave calculations for different models of the electronic ground state. The data are described very well by the Goodenough model, which has weakly interacting ferromagnetic zig-zag chains in the CE-type arrangement. A model that allows ferromagnetic dimers to form within the zigzags is inconsistent with the data. The analysis conclusively rules out the strongly bound dimer (Zener polaron) model.
我们已经测量了半掺杂双层锰酸盐 Pr(Ca,Sr)(2)Mn(2)O(7) 在其自旋、电荷和轨道有序相中自旋波谱。这些测量扩展到整个布里渊区并涵盖了整个单磁子谱,与不同电子基态模型的自旋波计算进行了严格比较。数据与 Goodenough 模型非常吻合,该模型在 CE 型排列中有弱相互作用的铁磁之字形链。允许在之字形内形成铁磁二聚体的模型与数据不一致。分析明确排除了强束缚二聚体(Zener 极化子)模型。