Wallner A, Melber K, Merchel S, Ott U, Forstner O, Golser R, Kutschera W, Priller A, Steier P
University of Vienna, Faculty of Physics, VERA Laboratory, Währinger Strasse 17, A-1090 Vienna, Austria ; Department of Nuclear Physics, Research School of Physics and Engineering, The Australian National University, Canberra, Australia ; Australian Nuclear Science and Technology Organisation (ANSTO), Lucas Heights, Australia.
Nucl Instrum Methods Phys Res B. 2013 Jan;294(2-2):496-502. doi: 10.1016/j.nimb.2012.03.036.
Nanodiamonds are stardust grains commonly found in primitive meteorites. They survived the formation of the solar system and kept their own individuality. Measurements of trace-element isotopic signatures in these grains will help understanding heavy element nucleosynthesis in massive stars and dust formation from their ejecta. We have continued previous attempts to search for stable Pt isotope anomalies in nanodiamonds via trace element accelerator mass spectrometry (TEAMS). The installation of a new injector beam line at the VERA facility allowed studying low traces of stable elements in different materials. Moreover, recent experiments showed that VERA provides the required measurement precision together with a low Pt machine background. Here, we observed for the first time an indication for enhancements of Pt/Pt isotope ratios in two diamond residues prepared by different chemical separation techniques from the Allende meteorite. Variations in other isotopic ratios were within analytical uncertainty, and no anomaly was identified in a third diamond fraction.
纳米金刚石是常见于原始陨石中的星尘颗粒。它们历经太阳系的形成过程并保持了自身特性。对这些颗粒中微量元素同位素特征的测量将有助于理解大质量恒星中的重元素核合成以及由其喷发物质形成尘埃的过程。我们延续了之前通过微量元素加速器质谱法(TEAMS)在纳米金刚石中寻找稳定铂同位素异常的尝试。VERA设施上新安装的注入器束流线使得研究不同材料中的低含量稳定元素成为可能。此外,近期实验表明VERA能提供所需的测量精度以及较低的铂仪器本底。在此,我们首次观察到通过不同化学分离技术从阿连德陨石制备的两个金刚石残渣中铂/铂同位素比值升高的迹象。其他同位素比值的变化在分析不确定度范围内,并且在第三个金刚石组分中未发现异常。