Begy R Cs, Somlai J, Kovacs T, Dumitru Rusu O A, Cosma C
Faculty of Environmental and Engineering Science, Babes-Bolyai University, Cluj-Napoca, Romania.
Radiat Prot Dosimetry. 2013 Nov;157(1):120-4. doi: 10.1093/rpd/nct121. Epub 2013 May 7.
Due to the relatively high activity concentrations of (210)Po that are found in tobacco, cigarette smoking has been found to be the principal pathway of the intake of this radionuclide. The (210)Po concentrations in the lung tissues may contribute significantly to an increase in the internal radiation dose and in the number of instances of lung cancer observed among smokers. The study of (210)Po in tobacco is required due to its potential for human radiation exposure through ingestion and inhalation. The risk factor caused by (210)Po in Romanian commercial cigarettes is not yet evaluated. Ten of the most frequently smoked brands of cigarettes sold in Romania were investigated in this work for this purpose. The activity concentration of (210)Po was determined by alpha spectrometry using a PIPS detector after chemical leaching and spontaneous deposition of (210)Po on a stainless steel disc from diluted HCl solution. The samples were spiked with (209)Po for chemical recovery calculation. The (210)Po activity concentrations of the measured types of cigarettes ranged from 4.65 to 10.22 mBq sample(-1) and the resulted average concentration of (210)Po isotopes is 8.35±0.80 mBq cigarette(-1) (the errors form a 2σ interval of confidence). When comparing the results of this study with the activity concentration values reported by other countries it was found that the results of this study are in the lower end of the world range. The estimation of this study shows that cigarette smokers, who are smoking one pack (20 cigarettes) per day, are exposed to an effective dose of 75.51 μSv y(-1).
由于烟草中发现的(210)钋活度浓度相对较高,吸烟已被发现是摄入这种放射性核素的主要途径。肺组织中的(210)钋浓度可能会显著增加吸烟者体内的辐射剂量以及肺癌的发病例数。由于(210)钋有可能通过摄入和吸入对人体造成辐射暴露,因此需要对烟草中的(210)钋进行研究。罗马尼亚商业香烟中(210)钋所造成的风险因素尚未评估。为此,本研究调查了罗马尼亚最常被吸食的10个香烟品牌。采用PIPS探测器通过α能谱法测定(210)钋的活度浓度,具体操作是先进行化学浸出,然后使(210)钋从稀释的HCl溶液中自发沉积在不锈钢圆盘上。样品中加入(209)钋用于化学回收率计算。所测香烟类型的(210)钋活度浓度范围为4.65至10.22 mBq/样品,(210)钋同位素的平均浓度为8.35±0.80 mBq/香烟(误差形成2σ置信区间)。将本研究结果与其他国家报告的活度浓度值进行比较时发现,本研究结果处于全球范围的较低水平。本研究估计表明,每天吸食一包(20支)香烟的吸烟者所接受的有效剂量为75.51 μSv/y。