Department of Physics and Astronomy, Louisiana State University, Baton Rouge, LA 70803, USA.
Proc Natl Acad Sci U S A. 2013 Jun 4;110(23):9283-8. doi: 10.1073/pnas.1307113110. Epub 2013 May 20.
The attractive/repulsive relationship between superconductivity and magnetic ordering has fascinated the condensed matter physics community for a century. In the early days, magnetic impurities doped into a superconductor were found to quickly suppress superconductivity. Later, a variety of systems, such as cuprates, heavy fermions, and Fe pnictides, showed superconductivity in a narrow region near the border to antiferromagnetism (AFM) as a function of pressure or doping. However, the coexistence of superconductivity and ferromagnetic (FM) or AFM ordering is found in a few compounds [RRh4B4 (R = Nd, Sm, Tm, Er), R'Mo6X8 (R' = Tb, Dy, Er, Ho, and X = S, Se), UMGe (M = Ge, Rh, Co), CeCoIn5, EuFe2(As(1-x)P(x))2, etc.], providing evidence for their compatibility. Here, we present a third situation, where superconductivity coexists with FM and near the border of AFM in Fe(1-x)Pd(x)Te. The doping of Pd for Fe gradually suppresses the first-order AFM ordering at temperature T(N/S), and turns into short-range AFM correlation with a characteristic peak in magnetic susceptibility at T'(N). Superconductivity sets in when T'(N) reaches zero. However, there is a gigantic ferromagnetic dome imposed in the superconducting-AFM (short-range) cross-over regime. Such a system is ideal for studying the interplay between superconductivity and two types of magnetic (FM and AFM) interactions.
超导性和磁有序之间的吸引力/排斥关系吸引了凝聚态物理界一个世纪。在早期,人们发现掺杂到超导体中的磁性杂质会迅速抑制超导性。后来,各种系统,如铜酸盐、重费米子和 Fe 磷化物,在压力或掺杂的作用下,在反铁磁序(AFM)边界附近的狭窄区域显示出超导性。然而,在少数化合物中发现了超导性和铁磁(FM)或 AFM 有序的共存[RRh4B4(R = Nd、Sm、Tm、Er)、R'Mo6X8(R' = Tb、Dy、Er、Ho 和 X = S、Se)、UMGe(M = Ge、Rh、Co)、CeCoIn5、EuFe2(As(1-x)P(x))2 等],这为它们的兼容性提供了证据。在这里,我们提出了第三种情况,即在 Fe(1-x)Pd(x)Te 中,超导性与 FM 和 AFM 边界共存。Pd 对 Fe 的掺杂逐渐抑制了温度 T(N/S)下的一级 AFM 有序,并在磁性磁化率的特征峰 T'(N)处转变为短程 AFM 相关性。当 T'(N)达到零时,超导性开始出现。然而,在超导-AFM(短程)交叉过渡区域存在巨大的铁磁畴。这样的系统非常适合研究超导性和两种类型的磁(FM 和 AFM)相互作用之间的相互作用。