Department of Clinical Neuroscience, Psychiatry Section, Karolinska Institutet, Karolinska Hospital, S-17176 Stockholm, Sweden.
Nucl Med Biol. 2013 Aug;40(6):747-54. doi: 10.1016/j.nucmedbio.2013.05.007. Epub 2013 Jun 27.
Evaluation of the α1-adrenoceptors in relation to brain pathophysiology and drug treatment has been hindered by lack of α1-adrenoceptor specific radioligands with sufficient brain exposure. Our aim was to develop an α1-adrenoceptor specific PET radioligand for brain imaging.
Two sertindole analogues 1-(4-fluorophenyl)-5-(1-methyl-1H-1,2,4-triazol-3-yl)-3-(1-[(11)C]methylpiperidin-4-yl)-1H-indole [(11)C]3 and 1-(4-fluorophenyl)-3-(1-[(11)C]methylpiperidin-4-yl)-5-(pyrimidin-5-yl)-1H-indole ([(11)C]Lu AA27122) [(11)C]4 were synthesized and evaluated as α1-adrenoceptor PET radioligands in cynomolgus monkey. Compounds 3 and 4 were selected due to their promising in vitro preclinical profile; high affinity and selectivity for the α1-adrenoceptor, favourable blood brain barrier permeability rates in Caco-2 monolayers and promising brain tissue/plasma ratio, assessed by equilibrium dialysis of free fraction in plasma and brain homogenate.
Compounds [(11)C]3 and [(11)C]4 were synthesized from their desmethyl piperidine precursors with high specific radioactivity (>370 GBq/μmol) using [(11)C]methyl iodide. The 1,2,4-triazole analogue [(11)C]3 exhibited poor brain uptake, but the corresponding pyrimidyl analogue [(11)C]4 exhibited high brain exposure and binding in α1-adrenoceptor rich brain regions. However, the binding could not be inhibited by pretreatment with prazosin (0.1 mg/kg and 0.3 mg/kg). The results were extended by autoradiography of [(11)C]4 binding in human brain sections and competition with antagonists from different structural families, revealing that only a minor portion of the observed binding of [(11)C]4 in brain was α1-adrenoceptor specific.
Though [(11)C]3 and [(11)C]4 proved not suitable as PET radioligands, the study provided further understanding of structural features influencing brain exposure of the chemical class of compounds related to the antipsychotic drug sertindole. It provided valuable insight in the delicacy of blood brain barrier penetration for structurally related compounds and underlines the importance for improved protocols for evaluation of brain penetration of future PET ligands.
由于缺乏具有足够脑暴露量的α1-肾上腺素受体特异性放射性配体,因此评估与脑病理生理学和药物治疗有关的α1-肾上腺素受体受到了阻碍。我们的目的是开发用于脑成像的α1-肾上腺素受体特异性 PET 放射性配体。
我们合成了两种 sertindole 类似物 1-(4-氟苯基)-5-(1-甲基-1H-1,2,4-三唑-3-基)-3-(1-[(11)C]甲基哌啶-4-基)-1H-吲哚[11C]3 和 1-(4-氟苯基)-3-(1-[(11)C]甲基哌啶-4-基)-5-(嘧啶-5-基)-1H-吲哚([(11)C]Lu AA27122)[(11)C]4,并在食蟹猴中评估了它们作为α1-肾上腺素受体 PET 放射性配体的性能。由于它们具有有前景的体外临床前特性,因此选择了化合物 3 和 4:对α1-肾上腺素受体具有高亲和力和选择性、在 Caco-2 单层中具有有利的血脑屏障渗透率以及通过在血浆和脑匀浆中评估游离分数的平衡透析获得的有前途的脑组织/血浆比。
使用[(11)C]甲基碘化物从它们的去甲基哌啶前体合成了化合物[(11)C]3 和 [(11)C]4,具有高比活度(>370GBq/μmol)。1,2,4-三唑类似物[(11)C]3 的脑摄取较差,但相应的嘧啶类似物[(11)C]4 表现出高脑暴露和富含α1-肾上腺素受体的脑区结合。然而,用普萘洛尔(0.1mg/kg 和 0.3mg/kg)预处理不能抑制结合。通过对人类脑切片中[(11)C]4 结合的放射自显影和与来自不同结构家族的拮抗剂的竞争,进一步扩展了结果,结果表明,在脑内观察到的[(11)C]4 结合中,只有一小部分是α1-肾上腺素受体特异性的。
尽管[(11)C]3 和 [(11)C]4 不适合作为 PET 放射性配体,但该研究进一步了解了影响 sertindole 类抗精神病药物相关化合物脑暴露的结构特征。它为评估未来 PET 配体脑穿透性的改进方案提供了有价值的见解,并强调了对结构相关化合物血脑屏障穿透性的敏感性。