Škarabot M, Lokar Ž, Muševič I
J. Stefan Institute, Jamova 39, SI-1000 Ljubljana, Slovenia.
Phys Rev E Stat Nonlin Soft Matter Phys. 2013 Jun;87(6):062501. doi: 10.1103/PhysRevE.87.062501. Epub 2013 Jun 3.
We demonstrate manipulation and transport of microparticles and even fluorescent molecules by the thermally induced gradient of the order parameter in the nematic liquid crystal. We use IR light absorption of the tightly focused beam of laser tweezers to heat locally a thin layer of the nematic liquid crystal by several degrees. This creates a spatial gradient of temperature of the nematic liquid crystal over separations of several tens of micrometers. We show that a dipolar colloidal particle is attracted into the hot spot of the laser tweezers. The depth of the trapping potential scales linearly with particle radius, indicating that the trapping mechanism is due to elastic self-energy of the distorted nematic liquid crystal around the particle and softening of the elasticity with increased temperature of the liquid crystal. We also demonstrate that this thermal trapping mechanism is efficient down to the nanoscale, as fluorescent molecules are also transported into hotter regions of the liquid crystal. This effect is absent in the isotropic phase, which calls into question particle transport due to the Soret effect.
我们展示了通过向列相液晶中序参量的热致梯度来操控和运输微粒甚至荧光分子。我们利用激光镊子紧密聚焦光束的红外光吸收,将向列相液晶的一薄层局部加热几度。这在几十微米的间距上产生了向列相液晶的空间温度梯度。我们表明,一个偶极胶体粒子会被吸引到激光镊子的热点处。捕获势的深度与粒子半径呈线性比例关系,这表明捕获机制是由于粒子周围扭曲的向列相液晶的弹性自能以及随着液晶温度升高弹性的软化。我们还证明,这种热捕获机制在纳米尺度下也是有效的,因为荧光分子也会被运输到液晶的较热区域。在各向同性相中不存在这种效应,这对因索雷特效应导致的粒子运输提出了质疑。