Department of Physics, Engineering Physics and Astronomy, Queen's University, Kingston, Ontario, Canada.
Opt Lett. 2013 May 15;38(10):1691-3. doi: 10.1364/OL.38.001691.
Charge-neutral excitons in semiconductor quantum dots (QDs) have a small finite energy separation caused by the anisotropic exchange splitting. Coherent excitation of neutral excitons will generally excite both exciton components, unless the excitation is parallel to one of the dipole axes. We present a polaron master equation model to describe two-exciton pumping using a coherent continuous wave pump field in the presence of a realistic anisotropic exchange splitting. We predict a five-peak incoherent spectrum, namely a Mollow quintuplet under general excitation conditions. We experimentally confirm such spectral quintuplets for In(Ga)As QDs and obtain very good agreement with theory.
半导体量子点(QDs)中的中性激子由于各向异性交换劈裂而具有较小的有限能量分离。除非激发与偶极轴之一平行,否则中性激子的相干激发通常会激发两个激子分量。我们提出了一个极化子主方程模型,用于描述在存在实际各向异性交换劈裂的情况下使用相干连续波泵浦场的双激子泵浦。我们预测了一个五峰非相干光谱,即在一般激发条件下的一个 Mollow 五重线。我们实验证实了 In(Ga)As QDs 的这种光谱五重线,并与理论取得了非常好的一致。