Department of Chemistry and †Department of Electrical and Computer Engineering, Laboratory for Nanophotonics, Rice University , Houston, Texas 77005, United States.
Nano Lett. 2013 Oct 9;13(10):4779-84. doi: 10.1021/nl402358h. Epub 2013 Sep 16.
For integrating and multiplexing of subwavelength plasmonic waveguides with other optical and electric components, complex architectures such as junctions with sharp turns are necessary. However, in addition to intrinsic losses, bending losses severely limit plasmon propagation. In the current work, we demonstrate that propagation of surface plasmon polaritons around 90° turns in silver nanoparticle chains occurs without bending losses. Using a far-field fluorescence method, bleach-imaged plasmon propagation (BlIPP), which creates a permanent map of the plasmonic near-field through bleaching of a fluorophore coated on top of a plasmonic waveguide, we measured propagation lengths at 633 nm for straight and bent silver nanoparticle chains of 8.0 ± 0.5 and 7.8 ± 0.4 μm, respectively. These propagation lengths were independent of the input polarization. We furthermore show that subradiant plasmon modes yield a longer propagation length compared to energy transport via excitation of super-radiant modes.
为了将亚波长等离子体波导与其他光学和电学组件集成和复用,需要复杂的结构,例如具有急转弯的接头。然而,除了固有损耗之外,弯曲损耗严重限制了等离子体的传播。在当前的工作中,我们证明了在银纳米粒子链中,表面等离子体激元在 90°转弯处的传播不会产生弯曲损耗。我们使用远场荧光法,即通过在等离子体波导顶部涂覆的荧光团的漂白来创建等离子体近场的永久图的漂白成像等离子体传播(BlIPP),测量了在 633nm 下直的和弯曲的银纳米粒子链的传播长度,分别为 8.0±0.5μm 和 7.8±0.4μm。这些传播长度与输入偏振无关。我们还表明,与通过激发超辐射模式进行的能量传输相比,亚辐射等离子体模式产生了更长的传播长度。