Hai Ting-Ting, Chen Ying-Jun, Wang Yan, Tian Chong-Guo, Lin Tian
Key Laboratory of Coastal Zone Environmental Processes and Ecological Remediation, Shandong Provincial Key Laboratory of Coastal Zone Environmental Processes, Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences, Yantai 264003, China.
Huan Jing Ke Xue. 2013 Jul;34(7):2533-8.
As the emission source of polycyclic aromatic hydrocarbons (PAHs), domestic coal combustion has attracted increasing attention in China. According to the coal maturity, combustion form and stove type associated with domestic coal combustion, a large-size, full-flow dilution tunnel and fractional sampling system was employed to collect the emissions from five coals with various maturities, which were burned in the form of raw-coal-chunk (RCC)/honeycomb-coal-briquettes (HCB) in different residential stoves, and then the emission factors of PAHs (EF(PAHs)) were achieved. The results indicate that the EF(PAHs) of bituminous coal ranged from 1.1 mg x kg(-1) to 3.9 mg x kg(-1) for RCC and 2.5 mg x kg(-1) to 21. 1 mg x kg(-1) for HCB, and the anthracite EF(PAH8) were 0.2 mg x kg(-1) for RCC and 0.6 mg x kg(-1) for HCB, respectively. Among all the influence factors of emission factors of PAHs from domestic coal combustion, the maturity of coal played a major role, the range of variance reaching 1 to 2 orders of magnitude in coals with different maturity. Followed by the form of combustion (RCC/HCB), the EF(PAHs) of HCB was 2-6 times higher than that of RCC for the same geological maturity of the coal. The type of stove had little influence on EF(PAHs).
作为多环芳烃(PAHs)的排放源,家用煤燃烧在中国已引起越来越多的关注。根据与家用煤燃烧相关的煤成熟度、燃烧形式和炉灶类型,采用大型全流稀释风洞和分级采样系统,收集了五种不同成熟度的煤在不同家用炉灶中以原煤块(RCC)/蜂窝煤球(HCB)形式燃烧时的排放物,进而得出多环芳烃的排放因子(EF(PAHs))。结果表明,烟煤以RCC形式燃烧时的EF(PAHs)范围为1.1 mg x kg(-1)至3.9 mg x kg(-1),以HCB形式燃烧时为2.5 mg x kg(-1)至21.1 mg x kg(-1);无烟煤以RCC形式燃烧时的EF(PAH8)为0.2 mg x kg(-1),以HCB形式燃烧时为0.6 mg x kg(-1)。在所有影响家用煤燃烧多环芳烃排放因子的因素中,煤的成熟度起主要作用,不同成熟度煤的变化范围达1至2个数量级。其次是燃烧形式(RCC/HCB),对于相同地质成熟度的煤,HCB的EF(PAHs)比RCC高2至6倍。炉灶类型对EF(PAHs)影响较小。