State Key Laboratory of Precision Spectroscopy, Department of Physics, East China Normal University, Shanghai 200062, China.
Sensors (Basel). 2013 Aug 26;13(9):11350-61. doi: 10.3390/s130911350.
Localized surface plasmon resonances (LSPRs) in metallic nanostructures have been studied intensely in the last decade. Fano interference is an important way to decrease the resonance linewidth and enhance the spectral detection resolution, but realizing a Fano lineshape with both a narrow linewidth and high spectral contrast-ratio is still challenging. Here we propose a metallic nanostructure consisting of a concentric square ring-disk (CSRD) nanostructure and an outside nanorod. Fano linewidth and spectral contrast ratio can be actively manipulated by adjusting the gap between the nanorod and CSRD, and by adjusting the gap between the ring and disk in CSRD. When the gap size in CSRD is reduced to 5 nm, the quadrupolar Fano linewidth is of 0.025 eV, with a contrast ratio of 80%, and the figure of merit reaches 15.
在过去的十年中,金属纳米结构中的局域表面等离激元共振(LSPR)受到了强烈的研究。 菲诺干涉是减小共振线宽和提高光谱检测分辨率的重要途径,但是实现具有窄线宽和高光谱对比度比的菲诺线型仍然具有挑战性。 在这里,我们提出了一种由同心方环盘(CSRD)纳米结构和外部纳米棒组成的金属纳米结构。 通过调整纳米棒与 CSRD 之间的间隙以及 CSRD 中环与盘之间的间隙,可以主动控制 Fano 线宽和光谱对比度比。 当 CSRD 中的间隙尺寸减小到 5nm 时,四极 Fano 线宽为 0.025eV,对比度比为 80%,品质因数达到 15。