镁离子和水分子对无定形碳酸钙结构的影响:分子动力学研究。
Effects of magnesium ions and water molecules on the structure of amorphous calcium carbonate: a molecular dynamics study.
机构信息
National Institute of Advanced Industrial Science and Technology (AIST) , Onogawa 16-1, Tsukuba 305-8569, Japan.
出版信息
J Phys Chem B. 2013 Nov 27;117(47):14849-56. doi: 10.1021/jp407721x. Epub 2013 Nov 15.
Molecular dynamics simulations were conducted to elucidate the effects of Mg(2+) and H2O additives on the structure of amorphous calcium carbonate (ACC). New potential parameters for Mg(2+) ions were developed. The distribution function of the angle formed by three nearest-neighbor atoms was introduced to analyze the short-range local structure of ACC. The simulation indicated that ACC had a weakly ordered local structure resembling the local structure of a CaCO3 crystal. The local structure of pure ACC resembled that of vaterite. The formation of the vaterite-like local structure was hindered by Mg(2+) ions, whereas H2O molecules did not significantly influence the structure of ACC when the fraction of H2O molecules was low. However, when the fraction of H2O was high, the formation of a monohydrocalcite-like local structure was promoted. The effects of the additives on the structure of ACC were verified using the size of the additives and the interaction between the additives and CaCO3. The simulated structure of ACC was compared with the structure of CaCO3 crystals nucleated through the formation of ACC particles in real systems.
采用分子动力学模拟方法阐明了 Mg(2+)和 H2O 添加剂对无定形碳酸钙 (ACC) 结构的影响。为 Mg(2+)离子开发了新的势能参数。引入了由三个最近邻原子形成的角度分布函数来分析 ACC 的短程局部结构。模拟表明,ACC 具有类似于 CaCO3 晶体局部结构的弱有序局部结构。纯 ACC 的局部结构类似于文石。Mg(2+)离子阻碍了文石样局部结构的形成,而 H2O 分子在 H2O 分子分数较低时对 ACC 的结构没有显著影响。然而,当 H2O 分数较高时,促进了一水合碳酸钙样局部结构的形成。通过添加剂的大小和添加剂与 CaCO3 之间的相互作用验证了添加剂对 ACC 结构的影响。将模拟的 ACC 结构与通过真实体系中 ACC 颗粒形成成核的 CaCO3 晶体结构进行了比较。