Physikalisches Institut, Universität Heidelberg, 69120 Heidelberg, Germany.
Science. 2013 Nov 22;342(6161):954-6. doi: 10.1126/science.1244843. Epub 2013 Nov 7.
Electronically highly excited (Rydberg) atoms experience quantum state-changing interactions similar to Förster processes found in complex molecules, offering a model system to study the nature of dipole-mediated energy transport under the influence of a controlled environment. We demonstrate a nondestructive imaging method to monitor the migration of electronic excitations with high time and spatial resolution, using electromagnetically induced transparency on a background gas acting as an amplifier. The continuous spatial projection of the electronic quantum state under observation determines the many-body dynamics of the energy transport.
电子高度激发(里德伯)原子经历类似于复杂分子中发现的福斯特过程的量子态变化相互作用,为研究在受控环境影响下偶极介导能量传输的性质提供了一个模型系统。我们展示了一种非破坏性的成像方法,使用作为放大器的背景气体中的电磁感应透明,以高时间和空间分辨率监测电子激发的迁移。所观察的电子量子态的连续空间投影决定了能量传输的多体动力学。