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等离子体纳米天线与自组装 GaAs 量子点的十一纳米对准精度。

Eleven nanometer alignment precision of a plasmonic nanoantenna with a self-assembled GaAs quantum dot.

机构信息

Max Planck Institute for Solid State Research , Heisenbergstrasse 1, D-70569 Stuttgart, Germany.

出版信息

Nano Lett. 2014 Jan 8;14(1):197-201. doi: 10.1021/nl403730q. Epub 2013 Dec 19.

Abstract

Plasmonics offers the opportunity of tailoring the interaction of light with single quantum emitters. However, the strong field localization of plasmons requires spatial fabrication accuracy far beyond what is required for other nanophotonic technologies. Furthermore, this accuracy has to be achieved across different fabrication processes to combine quantum emitters and plasmonics. We demonstrate a solution to this critical problem by controlled positioning of plasmonic nanoantennas with an accuracy of 11 nm next to single self-assembled GaAs semiconductor quantum dots, whose position can be determined with nanometer precision. These dots do not suffer from blinking or bleaching or from random orientation of the transition dipole moment as colloidal nanocrystals do. Our method introduces flexible fabrication of arbitrary nanostructures coupled to single-photon sources in a controllable and scalable fashion.

摘要

等离子体激元学提供了一种对光与单量子发射器相互作用进行精细调控的机会。然而,等离子体激元的强场局域化要求的空间制造精度远远超出了其他纳米光子技术所需的精度。此外,为了将量子发射器和等离子体激元结合起来,这种精度必须在不同的制造工艺中实现。我们通过将等离子体纳米天线以 11nm 的精度精确地定位在单个自组装 GaAs 半导体量子点旁边,解决了这个关键问题,而量子点的位置可以达到纳米级的精度。这些量子点不会像胶体纳米晶体那样出现闪烁、漂白或跃迁偶极子随机取向的问题。我们的方法以可控和可扩展的方式,将任意纳米结构的灵活制造与单光子源结合在一起。

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