de Carvalho Luciana L, Maltarollo Vinícius G, de Lima Emmanuela Ferreira, Weber Karen C, Honorio Kathia M, da Silva Albérico B F
Instituto de Química de São Carlos, Universidade de São Paulo, São Carlos, Brazil.
Centro de Ciências Naturais e Humanas, Universidade Federal do ABC, Santo André, Brazil.
PLoS One. 2014 Jan 8;9(1):e81301. doi: 10.1371/journal.pone.0081301. eCollection 2014.
Among several biological targets to treat AIDS, HIV integrase is a promising enzyme that can be employed to develop new anti-HIV agents. The aim of this work is to propose a mechanistic interpretation of HIV-1 integrase inhibition and to rationalize the molecular features related to the binding affinity of studied ligands. A set of 79 HIV-1 integrase inhibitors and its relationship with biological activity are investigated employing 2D and 3D QSAR models, docking analysis and DFT studies. Analyses of docking poses and frontier molecular orbitals revealed important features on the main ligand-receptor interactions. 2D and 3D models presenting good internal consistency, predictive power and stability were obtained in all cases. Significant correlation coefficients (r(2) = 0.908 and q(2)= 0.643 for 2D model; r(2)= 0.904 and q(2)= 0.719 for 3D model) were obtained, indicating the potential of these models for untested compounds. The generated holograms and contribution maps revealed important molecular requirements to HIV-1 IN inhibition and several evidences for molecular modifications. The final models along with information resulting from molecular orbitals, 2D contribution and 3D contour maps should be useful in the design of new inhibitors with increased potency and selectivity within the chemical diversity of the data.
在治疗艾滋病的多个生物学靶点中,HIV整合酶是一种有前景的酶,可用于开发新型抗HIV药物。这项工作的目的是对HIV-1整合酶抑制作用提出一种机理解释,并阐明与所研究配体结合亲和力相关的分子特征。利用二维和三维定量构效关系模型、对接分析和密度泛函理论研究,对一组79种HIV-1整合酶抑制剂及其与生物活性的关系进行了研究。对接构象和前沿分子轨道分析揭示了主要配体-受体相互作用的重要特征。在所有情况下均获得了具有良好内部一致性、预测能力和稳定性的二维和三维模型。得到了显著的相关系数(二维模型的r(2) = 0.908和q(2)= 0.643;三维模型的r(2)= 0.904和q(2)= 0.719),表明这些模型对未测试化合物具有潜力。生成的全息图和贡献图揭示了HIV-1整合酶抑制的重要分子要求以及分子修饰的若干证据。最终模型以及分子轨道、二维贡献和三维等高线图所得到的信息,应有助于在数据的化学多样性范围内设计出具有更高效力和选择性的新型抑制剂。