Atorf Bernhard, Mühlenbernd Holger, Muldarisnur Mulda, Zentgraf Thomas, Kitzerow Heinz
Department of Chemistry, Faculty of Science, University of Paderborn, Warburger Str. 100, 33098 Paderborn (Germany), Fax: (+49) 5251 60 42 08; Center for Optoelectronics and Photonics Paderborn (CeOPP), University of Paderborn, Warburger Str. 100, 33098 Paderborn (Germany).
Chemphyschem. 2014 May 19;15(7):1470-6. doi: 10.1002/cphc.201301069. Epub 2014 Jan 31.
A metasurface comprising a two-dimensional array of split-ring resonators with resonance frequencies in the near-infrared region is fabricated and embedded in a uniformly aligned liquid crystal. The change of the dielectric permittivity in proximity to the plasmonic structure by the replacement of air with the liquid crystal results in a decrease in resonance frequencies. The resonance shift can be attributed to the interaction of the evanescent field of the excited resonant plasmon modes with the liquid crystal. This shift in resonance frequency is found to depend on the liquid-crystal alignment and to vary for different modes. Also, the resulting effects of changes in temperature or applied external electric field on the metasurface depend on the liquid-crystal alignment and may differ from mode to mode. These observations indicate that the characteristic frequencies of the resonant split-ring resonator modes may depend on different evanescent field components interacting with the liquid crystal. Consequently, certain design rules should be taken into account for the development of tunable metasurfaces based on liquid crystals.
制造了一种超表面,其由具有近红外区域共振频率的二维裂环谐振器阵列组成,并嵌入均匀排列的液晶中。用液晶取代空气导致靠近等离子体结构处的介电常数发生变化,从而使共振频率降低。共振频率的偏移可归因于激发的共振等离子体模式的倏逝场与液晶的相互作用。发现这种共振频率的偏移取决于液晶的排列,并且对于不同模式会有所变化。此外,温度变化或施加的外部电场对超表面产生的影响取决于液晶的排列,并且可能因模式而异。这些观察结果表明,共振裂环谐振器模式的特征频率可能取决于与液晶相互作用的不同倏逝场分量。因此,在开发基于液晶的可调谐超表面时应考虑某些设计规则。