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阿根廷中部半干旱地区(7)Be 土壤蓄积量的年际变化。

Annual variation of (7)Be soil inventory in a semiarid region of central Argentina.

机构信息

Grupo de Estudios Ambientales, Instituto de Matemática Aplicada San Luis, Universidad Nacional de San Luis - CONICET, Ejército de los Andes 950, D5700HHW San Luis, Argentina.

Grupo de Estudios Ambientales, Instituto de Matemática Aplicada San Luis, Universidad Nacional de San Luis - CONICET, Ejército de los Andes 950, D5700HHW San Luis, Argentina.

出版信息

J Environ Radioact. 2014 Apr;130:72-7. doi: 10.1016/j.jenvrad.2014.01.006. Epub 2014 Jan 31.

Abstract

Reliable information on environmental radionuclides atmospheric entrance, and their distribution along the soil profile, is a necessary condition for using these soil and sediment tracers to investigate key environmental processes. To address this need, (7)Be content in rainwater and the wet deposition in a semiarid region at San Luis Province, Argentina, were studied. Following these researches, in the same region, we have assessed the (7)Be content along a soil profile, during 2.5 years from September 2009 to January 2012. As expected, the specific activity values in soil samples in the wet period (November-April) were higher than in the dry period (May-October). During the investigated period (2009 - beginning 2012) and for all sampled points, the maximum value of the (7)Be specific activity (Bq kg(-1)) was measured at the surface level. A typical decreasing exponential function of (7)Be areal activity (Bq m(-2)) with soil mass depth (kg m(-2)) was found and the key distribution parameters were determined for each month. The minimum value of areal activity was 51 Bq m(-2) in August, and the maximum was 438 Bq m(-2) in February. The relaxation mass depth ranges from 2.9 kg m(-2) in March to 1.3 kg m(-2) in August. (7)Be wet deposition can explain in a very significant proportion the (7)Be inventory in soil. During the period of winds in the region (September and October), the (7)Be content in soil was greater than the expected contribution from wet deposition, situation that is compatible with a higher relative contribution of dry deposition at this period of the year.

摘要

可靠的环境放射性核素大气进入及其沿土壤剖面分布的信息,是利用这些土壤和沉积物示踪剂来研究关键环境过程的必要条件。为了满足这一需求,我们研究了阿根廷圣路易斯省半干旱地区雨水和湿沉降中的(7)Be 含量。在这些研究之后,我们在同一地区评估了 2009 年 9 月至 2012 年 1 月期间沿土壤剖面的(7)Be 含量。正如预期的那样,在湿期(11 月至 4 月),土壤样本中的比活度值高于干期(5 月至 10 月)。在调查期间(2009 年至 2012 年初)和所有采样点,(7)Be 比活度的最大值(Bq kg(-1))在地表水平测量。发现了(7)Be 面活性(Bq m(-2))与土壤质量深度(kg m(-2))的典型递减指数函数,并确定了每个月的关键分布参数。面活性的最小值为 51 Bq m(-2),最大值为 438 Bq m(-2)。在 3 月,松弛质量深度范围为 2.9 kg m(-2)至 8 月的 1.3 kg m(-2)。(7)Be 湿沉降可以在很大程度上解释土壤中(7)Be 的含量。在该地区(9 月和 10 月)有风期间,土壤中的(7)Be 含量大于湿沉降的预期贡献,这种情况与当年该时期干沉降的相对贡献较高是一致的。

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