Ding Chengyuan, Xiong Wei, Fan Tingting, Hickstein Daniel D, Popmintchev Tenio, Zhang Xiaoshi, Walls Mike, Murnane Margaret M, Kapteyn Henry C
Opt Express. 2014 Mar 10;22(5):6194-202. doi: 10.1364/OE.22.006194.
We demonstrate the highest flux tabletop source of coherent soft X-rays to date, driven by a single-stage 10 mJ Ti:sapphire regenerative amplifier at 1 kHz. We first down-convert the laser to 1.3 µm using a parametric amplifier, before up-converting it to soft X-rays using high harmonic generation in a high-pressure, phase matched, hollow waveguide geometry. The resulting optimally phase matched broadband spectrum extends to 200 eV, with a soft X-ray photon flux of > 10(6) photons/pulse/1% bandwidth at 1 kHz, corresponding to > 10(9) photons/s/1% bandwidth, or approximately a three order-of-magnitude increase compared with past work. Finally, using this broad bandwidth X-ray source, we demonstrate X-ray absorption spectroscopy of multiple elements and transitions in molecules in a single spectrum, with a spectral resolution of 0.25 eV, and with the ability to resolve the near edge fine structure.
我们展示了迄今为止通量最高的桌面式相干软X射线源,由一台1千赫兹的单级10毫焦钛宝石再生放大器驱动。我们首先使用参量放大器将激光下转换至1.3微米,然后在高压、相位匹配的空心波导结构中利用高次谐波产生将其升频转换为软X射线。由此产生的最佳相位匹配宽带光谱延伸至200电子伏特,在1千赫兹时软X射线光子通量>10⁶光子/脉冲/1%带宽,相当于>10⁹光子/秒/1%带宽,与过去的工作相比增加了约三个数量级。最后,使用这个宽带X射线源,我们在单个光谱中展示了多种元素和分子跃迁的X射线吸收光谱,光谱分辨率为0.25电子伏特,并且能够分辨近边精细结构。