Chemphyschem. 2014 Mar 17;15(4):619-29. doi: 10.1002/cphc.201300826.
This Minireview presents an overview of near-field hyperspectral imaging and discusses its applications. Based on a fibre-tip probe, the hyperspectral near-field optical microscope allows the simultaneous acquisition of near-field images over a broad spectral range (400 to 1000 nm), enabling the recovery of local spectroscopic information, which is essential for understanding the resonant interaction of light with nanostructured objects because the far-field and near-field spectral responses can differ significantly, as is the case for plasmonic nanostructures. The optical information is collected through local interactions with the evanescent fields at the surface of the sample; therefore, the approach provides spectroscopic information with nanoscale spatial resolution. Several applications of spectroscopic near-field microscopy are described for the visualisation of plasmonic modes in metallic nanostructures and near-field fluorescence spectroscopy.
这篇综述介绍了近场光谱成像技术,并讨论了其应用。基于光纤探针,近场光学显微镜能够在较宽的光谱范围内(400 至 1000nm)同时获取近场图像,从而恢复局部光谱信息,这对于理解光与纳米结构物体的共振相互作用至关重要,因为在等离子体纳米结构的情况下,远场和近场光谱响应可能有很大差异。光学信息通过与样品表面的消逝场的局部相互作用来收集;因此,该方法提供了具有纳米级空间分辨率的光谱信息。本文还介绍了几种光谱近场显微镜的应用,用于可视化金属纳米结构中的等离子体模式和近场荧光光谱。