Viamet Pharmaceuticals, Inc., Durham, NC 27703, USA.
Viamet Pharmaceuticals, Inc., Durham, NC 27703, USA.
Bioorg Med Chem Lett. 2014 Jun 1;24(11):2444-7. doi: 10.1016/j.bmcl.2014.04.024. Epub 2014 Apr 16.
The orally-active CYP17A1 inhibitor abiraterone acetate (AA) decreases adrenal and intratumoral androgen biosynthesis and is an effective agent for the treatment of prostate cancer. Abiraterone potently inhibits both reactions catalyzed by CYP17, the 17α-hydroxylase (hydroxylase) reaction as well as the 17,20-lyase (lyase) transformation. CYP17 hydroxylase inhibition prevents the synthesis of adrenal glucocorticoids and causes an accumulation of circulating mineralocorticoids. As a consequence of potent CYP17 hydroxylase inhibition (i.e., lack of lyase selectivity), AA must be co-administered with the cortisol replacement prednisone and patients may experience the effects of mineralocorticoid excess syndrome (MES). Herein, we describe rationally-designed, CYP17 lyase-selective inhibitors that could prove safer and more effective than abiraterone. Using proprietary methodology, the high-affinity pyridine or imidazole metal-binding group found in current clinical CYP17 inhibitors was replaced with novel, less avid, metal-binding groups in concert with potency-enhancing molecular scaffold modifications. This process produced a unique series of CYP17 lyase-selective inhibitors that included the oral agent 6 (VT-464), now in Phase 2 prostate cancer clinical trials. The chemical methodology described is potentially applicable to the design of new and more effective metalloenzyme inhibitor treatments for a broad array of diseases.
口服活性 CYP17A1 抑制剂醋酸阿比特龙(AA)可降低肾上腺和肿瘤内雄激素的生物合成,是治疗前列腺癌的有效药物。阿比特龙可强烈抑制 CYP17 催化的两种反应,即 17α-羟化酶(羟化酶)反应和 17,20-裂合酶(裂合酶)转化。CYP17 羟化酶抑制可阻止肾上腺糖皮质激素的合成,并导致循环中盐皮质激素的积累。由于强烈的 CYP17 羟化酶抑制(即缺乏裂合酶选择性),AA 必须与皮质醇替代泼尼松联合使用,患者可能会出现盐皮质激素过多综合征(MES)的影响。在此,我们描述了合理设计的、CYP17 裂合酶选择性抑制剂,它们可能比阿比特龙更安全、更有效。使用专有的方法,在当前临床 CYP17 抑制剂中发现的高亲和力吡啶或咪唑金属结合基团被新型、亲和力较低的金属结合基团取代,同时进行增强效力的分子支架修饰。该过程产生了一系列独特的 CYP17 裂合酶选择性抑制剂,包括口服药物 6(VT-464),目前正在进行前列腺癌的 2 期临床试验。所描述的化学方法在设计用于广泛疾病的新型和更有效的金属酶抑制剂治疗方面具有潜在的适用性。