1] The Advanced Photon Source, Argonne National Laboratory, Argonne, Illinois 60439, USA [2] The James Franck Institute and Department of Physics, University of Chicago, Chicago, Illinois 60637, USA.
The James Franck Institute and Department of Physics, University of Chicago, Chicago, Illinois 60637, USA.
Nat Commun. 2014 Jun 18;5:4218. doi: 10.1038/ncomms5218.
Pressure can transform a transparent material into an opaque one, quench the moments in a magnet and force solids to flow like liquids. At 15 GPa, the pressure found 500 km below the earth's surface, the semiconductors silicon and germanium superconduct. Yet, at this same pressure, we show here that the magnetism in metallic GdSi remains completely robust even as it shrinks by one-seventh of its volume. Non-resonant X-ray magnetic diffraction in a specially designed diamond anvil cell, combined with band structure calculations, reveal the stability of the incommensurate spin density wave, which can be traced to a persistently nested portion of the Fermi surface that becomes increasingly one-dimensional under pressure. A cooperative interaction between nested, itinerant spins and local magnetic moments provides the organizing principle for the modulated magnetic order, salient both for its insights into the role of topology in ordered states and its potential functionality.
压力可以使透明材料变成不透明材料,使磁铁中的瞬间消失,并使固体像液体一样流动。在地球表面以下 500 公里处发现的 15GPa 压力下,半导体硅和锗会超导。然而,在这里我们表明,即使在体积缩小七分之一的情况下,金属 GdSi 中的磁性仍然完全稳定。在专门设计的金刚石压腔中进行的非共振 X 射线磁衍射,结合能带结构计算,揭示了非调谐自旋密度波的稳定性,这可以追溯到费米面的一个持续嵌套部分,在压力下变得越来越一维。嵌套的、巡游的自旋和局部磁矩之间的协同相互作用为调制磁有序提供了组织原则,这对于理解拓扑在有序态中的作用及其潜在功能都很重要。