Groskreutz Stephen R, Weber Stephen G
Department of Chemistry, University of Pittsburgh, 219 Parkman Avenue, Pittsburgh, PA 15260, United States.
Department of Chemistry, University of Pittsburgh, 219 Parkman Avenue, Pittsburgh, PA 15260, United States.
J Chromatogr A. 2014 Aug 8;1354:65-74. doi: 10.1016/j.chroma.2014.05.056. Epub 2014 May 28.
Solvent-based on-column focusing is a powerful and well known approach for reducing the impact of pre-column dispersion in liquid chromatography. Here we describe an orthogonal temperature-based approach to focusing called temperature-assisted on-column solute focusing (TASF). TASF is founded on the same principles as the more commonly used solvent-based method wherein transient conditions are created that lead to high solute retention at the column inlet. Combining the low thermal mass of capillary columns and the temperature dependence of solute retention TASF is used effectively to compress injection bands at the head of the column through the transient reduction in column temperature to 5°C for a defined 7mm segment of a 6cm long 150μm I.D. column. Following the 30s focusing time, the column temperature is increased rapidly to the separation temperature of 60°C releasing the focused band of analytes. We developed a model to simulate TASF separations based on solute retention enthalpies, focusing temperature, focusing time, and column parameters. This model guides the systematic study of the influence of sample injection volume on column performance. All samples have solvent compositions matching the mobile phase. Over the 45-1050nL injection volume range evaluated, TASF reduces the peak width for all solutes with k' greater than or equal to 2.5, relative to controls. Peak widths resulting from injection volumes up to 1.3 times the column fluid volume with TASF are less than 5% larger than peak widths from a 45nL injection without TASF (0.07 times the column liquid volume). The TASF approach reduced concentration detection limits by a factor of 12.5 relative to a small volume injection for low concentration samples. TASF is orthogonal to the solvent focusing method. Thus, it can be used where on-column focusing is required, but where implementation of solvent-based focusing is difficult.
基于溶剂的柱上聚焦是一种强大且广为人知的方法,用于减少液相色谱中柱前扩散的影响。在此,我们描述一种基于温度的正交聚焦方法,称为温度辅助柱上溶质聚焦(TASF)。TASF基于与更常用的基于溶剂的方法相同的原理,即创造瞬态条件,导致柱入口处溶质保留率高。结合毛细管柱的低热质量和溶质保留的温度依赖性,TASF通过将6cm长、内径150μm的柱的特定7mm段的柱温度瞬态降至5°C,有效地用于压缩柱前端的进样带。在30s的聚焦时间后,柱温度迅速升至60°C的分离温度,释放被聚焦的分析物带。我们开发了一个模型,基于溶质保留焓、聚焦温度、聚焦时间和柱参数来模拟TASF分离。该模型指导对进样体积对柱性能影响的系统研究。所有样品的溶剂组成与流动相匹配。在所评估的45 - 1050nL进样体积范围内,相对于对照,TASF减小了所有k'大于或等于2.5的溶质的峰宽。对于TASF,进样体积高达柱流体体积1.3倍时产生的峰宽,比无TASF的45nL进样(0.07倍柱液体体积)产生的峰宽仅大不到5%。对于低浓度样品,TASF方法相对于小体积进样将浓度检测限降低了12.5倍。TASF与溶剂聚焦方法正交。因此,在需要柱上聚焦但难以实施基于溶剂的聚焦的情况下可以使用它。