Chen Zuxin, Lai Boya, Zhang Junming, Wang Guoping, Chu Sheng
State Key Laboratory for Optoelectronics Materials and Technology, Sun Yat-sen University, Guangzhou, People's Republic of China, 510275.
Nanotechnology. 2014 Jul 25;25(29):295203. doi: 10.1088/0957-4484/25/29/295203. Epub 2014 Jul 3.
Plasmonic noble metal nanodisks with regular (triangular or hexagonal) shapes have been epitaxially formed on ZnO nanorods' (0002) surfaces. The composite material's crystal structures, epitaxial relationships between metal nanodisks, and ZnO host crystals were fully investigated. The effects from metal nanodisks on lasing characteristics of two types of ZnO nanoscale cavities (Fabry-Perot and Whispering Gallery Mode cavity) were studied. The results suggest that metal nanodisks can effectively enhance the lasing performance by lowering the lasing threshold in the ZnO Whispering Gallery Mode nanoplate laser, whereas the Fabry-Perot ZnO nanorods lasers were much less affected by the metal decoration. The plasmonic enhancement mechanism for the ZnO nanoplate cavities was further studied using numerical simulations as well as spatially resolved photoluminescence measurement.
具有规则(三角形或六边形)形状的等离子体贵金属纳米盘已在ZnO纳米棒的(0002)表面上外延形成。对该复合材料的晶体结构、金属纳米盘与ZnO主体晶体之间的外延关系进行了全面研究。研究了金属纳米盘对两种类型的ZnO纳米级腔(法布里-珀罗腔和回音壁模腔)激光特性的影响。结果表明,金属纳米盘可通过降低ZnO回音壁模纳米板激光器的激光阈值来有效提高激光性能,而法布里-珀罗ZnO纳米棒激光器受金属修饰的影响要小得多。利用数值模拟以及空间分辨光致发光测量进一步研究了ZnO纳米板腔的等离子体增强机制。