RIKEN Center for Emergent Matter Science (CEMS), Wako, Saitama 351-0198, Japan.
RIKEN Center for Emergent Matter Science (CEMS), Wako, Saitama 351-0198, Japan and Department of Applied Physics, University of Tokyo, Tokyo 113-8656, Japan.
Phys Rev Lett. 2014 Jun 20;112(24):246402. doi: 10.1103/PhysRevLett.112.246402. Epub 2014 Jun 18.
Because of the recent development of thin film and artificial superstructure growth techniques, it is possible to control the dimensionality of the system, smoothly between two and three dimensions. In this Letter we unveil the dimensional crossover of emergent topological phenomena in correlated topological materials. In particular, by focusing on the thin film of pyrochlore iridate antiferromagnets grown along the [111] direction, we demonstrate that the thin film can have a giant anomalous Hall conductance, proportional to the thickness of the film, even though there is no Hall effect in 3D bulk material. Moreover, in the case of ultrathin films, a quantized anomalous Hall conductance can be observed, despite the fact that the system is an antiferromagnet. In addition, we uncover the emergence of a new topological phase, the nontrivial topological properties of which are hidden in the bulk insulator and manifest only in thin films. This shows that the thin film of correlated topological materials is a new platform to search for unexplored novel topological phenomena.
由于近年来薄膜和人工超结构生长技术的发展,人们有可能在二维和三维之间平滑地控制系统的维度。在这封信中,我们揭示了关联拓扑材料中新兴拓扑现象的维度交叉。具体来说,通过关注沿[111]方向生长的钙钛矿碘氧化物反铁磁体的薄膜,我们证明了尽管在 3D 体材料中没有霍尔效应,但薄膜可以具有与薄膜厚度成正比的巨大反常霍尔电导率。此外,在超薄薄膜的情况下,尽管系统是反铁磁体,仍可以观察到量化的反常霍尔电导率。此外,我们揭示了一种新的拓扑相的出现,其拓扑性质在体绝缘材料中是隐藏的,仅在薄膜中表现出来。这表明关联拓扑材料的薄膜是一个新的平台,可以探索尚未探索的新拓扑现象。