Department of Physics, Renmin University of China, Beijing 100872, China.
School of Energy, Power and Mechanical Engineering, North China Electric Power University, Beijing 102206, China.
Phys Rev Lett. 2013 Sep 6;111(10):107004. doi: 10.1103/PhysRevLett.111.107004. Epub 2013 Sep 4.
We present a high-pressure NMR study of the overdoped iron pnictide superconductor NaFe0.94Co0.06As. The low-energy antiferromagnetic spin fluctuations in the normal state, manifest as the Curie-Weiss upturn in the spin-lattice relaxation rate 1/(75)T1T, first increase strongly with pressure but fall again at P>Popt=2.2 GPa. Neither long-ranged magnetic order nor a structural phase transition is encountered up to 2.5 GPa. The superconducting transition temperature Tc shows a pressure dependence identical to the spin fluctuations. Our observations demonstrate that magnetic correlations and superconductivity are optimized simultaneously as a function of the electronic structure, thereby supporting very strongly a magnetic origin of superconductivity.
我们呈现了高压 NMR 研究过掺杂铁砷化物超导体 NaFe0.94Co0.06As 的结果。正常态下的低能反铁磁自旋涨落表现为自旋晶格弛豫率 1/(75)T1T 的居里-外斯上翘,首先随压力急剧增加,但在 P>Popt=2.2 GPa 时再次下降。在 2.5 GPa 之前,既没有长程磁有序也没有结构相变。超导转变温度 Tc 表现出与自旋涨落相同的压力依赖性。我们的观察结果表明,磁关联和超导性作为电子结构的函数同时得到优化,从而强烈支持超导性的磁起源。