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区域污染事件期间利用地面和卫星遥感对背景站气溶胶光学特性及辐射强迫的观测研究

[Observation study on aerosol optical properties and radiative forcing using the ground-based and satellite remote sensing at background station during the regional pollution episodes].

作者信息

Zhang Xiao-Ling, Xia Xiang-Ao, Che Hui-Zheng, Tang Jie, Tang Yi-Xi, Meng Wei, Dong Fan

出版信息

Huan Jing Ke Xue. 2014 Jul;35(7):2439-48.

PMID:25247232
Abstract

The significant effect of anthropogenic pollutants transportation on the physical and optical properties of regional background atmospheric aerosol was studied by using ground-based and satellite remote sensing data obtained at the atmospheric background station (Shangdianzi, Beijing) of North China during October 1 to 15 in 2011. The aerosol mass concentration and reactive gases concentration increased obviously during periods of October 4-5, October 7-9, and October 11-12. Comparing with the background period of October 1-3, volume concentration increased by a factor of 3-6 for reactive gases such as NO(x), and CO, and a factor of 10-20 for SO2. Mass concentration of PM2.5 was about 200 microg x m(-3) on October 9. During haze period, the AOD at 500 nm varied between 0.60 to 1.00. The single scattering albedo (SSA) was lower than 0.88. And the black carbon concentration increased 4-8 times, which suggested the aerosol absorption was very strong during this pollution episode. The absorption of aerosol particles could cause 100-400 W x m(-2) increase of atmospheric radiation. The surface radiation decreased by about 100-300 W x m(-2) due to the aerosol scattering and absorption. This could cause higher stability of atmosphere, which will significantly affect the cloud and precipitation, and thus the regional weather and climate.

摘要

利用2011年10月1日至15日在中国北方大气本底站(北京上甸子)获取的地基和卫星遥感数据,研究了人为污染物传输对区域本底大气气溶胶物理和光学特性的显著影响。在10月4 - 5日、10月7 - 9日和10月11 - 12日期间,气溶胶质量浓度和活性气体浓度明显增加。与10月1 - 3日的本底期相比,NO(x)、CO等活性气体的体积浓度增加了3 - 6倍,SO2增加了10 - 20倍。10月9日PM2.5的质量浓度约为200μg x m(-3)。在雾霾期间,500nm处的气溶胶光学厚度(AOD)在0.60至1.00之间变化。单次散射反照率(SSA)低于0.88。黑碳浓度增加了4 - 8倍,这表明在这次污染事件中气溶胶吸收非常强烈。气溶胶颗粒的吸收可导致大气辐射增加100 - 400W x m(-2)。由于气溶胶的散射和吸收,地表辐射减少了约100 - 300W x m(-2)。这可能导致大气稳定性增加,从而显著影响云和降水,进而影响区域天气和气候。

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