1] Department of Physics &Astronomy, University of Pittsburgh, 3941 O'Hara Street, Pittsburgh, Pennsylvania 15260, USA [2] Pittsburgh Quantum Institute, Pittsburgh, Pennsylvania 15260, USA.
Department of Materials Science and Engineering, University of Wisconsin-Madison, Madison, Wisconsin 53706, USA.
Nat Commun. 2014 Sep 25;5:5019. doi: 10.1038/ncomms6019.
Reports of emergent conductivity, superconductivity and magnetism have helped to fuel intense interest in the rich physics and technological potential of complex-oxide interfaces. Here we employ magnetic force microscopy to search for room-temperature magnetism in the well-studied LaAlO3/SrTiO3 system. Using electrical top gating to control the electron density at the oxide interface, we directly observe the emergence of an in-plane ferromagnetic phase as electrons are depleted from the interface. Itinerant electrons that are reintroduced into the interface align antiferromagnetically with the magnetization at first screening and then destabilizing it as the conductive regime is approached. Repeated cycling of the gate voltage results in new, uncorrelated magnetic patterns. This newfound control over emergent magnetism at the interface between two non-magnetic oxides portends a number of important technological applications.
报告中出现的导电机理、超导和磁性现象,激发了人们对复杂氧化物界面丰富物理性质和潜在技术应用的强烈兴趣。在这项研究中,我们采用磁力显微镜,在 LaAlO3/SrTiO3 体系这一研究热点中,寻找室温磁性现象。通过对氧化物界面电子密度的电学门控,我们直接观察到当电子从界面耗尽时,出现了面内铁磁相。首先,进入界面的巡游电子与磁化强度反铁磁耦合,当进入导电态时,又使磁化强度失稳。门电压的重复循环导致新的、不相关的磁图案出现。这种对两种非磁性氧化物界面中出现的磁性的新控制,预示着许多重要的技术应用。