Schrader Frederik, Brümmer Christian
Thünen Institute of Climate-Smart Agriculture, Bundesallee 50, 38116 Braunschweig, Germany.
Water Air Soil Pollut. 2014;225(10):2114. doi: 10.1007/s11270-014-2114-7. Epub 2014 Sep 13.
Land use specific deposition velocities of atmospheric trace gases and aerosols-particularly of reactive nitrogen compounds-are a fundamental input variable for a variety of deposition models. Although the concept is known to have shortcomings-especially with regard to bi-directional exchange-the often limited availability of concentration data and meteorological input variables make it a valuable simplification for regional modeling of deposition fluxes. In order to meet the demand for an up-to-date overview of recent publications on measurements and modeling studies, we compiled a database of ammonia (NH) deposition velocities published from 2004 to 2013. Observations from a total of 42 individual studies were averaged using an objective weighing scheme and classified into seven land use categories. Weighted average and median deposition velocities are 2.2 and 2.1 cm s for coniferous forests, 1.5 and 1.2 cm s for mixed forests, 1.1 and 0.9 cm s for deciduous forests, 0.9 and 0.7 cm s for semi-natural sites, 0.7 and 0.8 cm s for urban sites, 0.7 and 0.6 cm s for water surfaces, and 1.0 and 0.4 cm s for agricultural sites, respectively. Thus, values presented in this compilation were considerably lower than those found in former studies (e.g., VDI 2006). Reasons for the mismatch were likely due to different land use classification, different averaging methods, choices of measurement locations, and improvements in measurement and in modeling techniques. Both data and code used for processing are made available as supplementary material to this article.
大气痕量气体和气溶胶(特别是活性氮化合物)的土地利用特定沉降速度是各种沉降模型的基本输入变量。尽管已知该概念存在缺陷,尤其是在双向交换方面,但浓度数据和气象输入变量的可用性通常有限,这使其成为区域沉降通量建模的一种有价值的简化方法。为了满足对近期测量和建模研究出版物最新综述的需求,我们汇编了一个2004年至2013年发表的氨(NH₃)沉降速度数据库。使用客观加权方案对总共42项独立研究的观测数据进行平均,并分为七种类别。针叶林的加权平均沉降速度和中值沉降速度分别为2.2和2.1厘米/秒,混交林为1.5和1.2厘米/秒,落叶林为1.1和0.9厘米/秒,半自然场地为0.9和0.7厘米/秒,城市场地为0.7和0.8厘米/秒,水面为0.7和0.6厘米/秒,农业场地为1.0和0.4厘米/秒。因此,本汇编中给出的值远低于以前研究中发现的值(例如VDI 2006)。不匹配的原因可能是由于土地利用分类不同、平均方法不同、测量地点的选择以及测量和建模技术的改进。处理所用的数据和代码均作为本文的补充材料提供。