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大气中二氧化氮和氨沉降至中国东南部一个典型农业生态系统的情况。

Atmospheric NO2 and NH3 deposition into a typical agro-ecosystem in Southeast China.

作者信息

Cui Jian, Zhou Jing, Yang Hao, Peng Ying, He Yuanqiu, Chan Andy

机构信息

Red soil ecological experiment station, Chinese Academy of Sciences, Liujiazhan plantation, Yingtan, P.R. China 335211.

出版信息

J Environ Monit. 2011 Nov;13(11):3216-21. doi: 10.1039/c1em10284b. Epub 2011 Oct 10.

Abstract

The dry deposition of atmospheric nitrogen (including NO(2) and NH(3)) into a typical agro-ecosystem in Southeast China during 2006-2007 was estimated. Results indicated that the dry deposition velocities of NO(2) and NH(3) ranged from 0.04-0.24 cm s(-1) and 0.09-0.47 cm s(-1), respectively. The higher values appeared in the non-crop growing period. Concentrations of atmospheric NO(2) and NH(3) ranged from 24.64-104.10 μgN m(-3) and 14.40-389.6 μgN m(-3), respectively. Variation of the NH(3) mixing ratio showed a clear double-peak. NO(2) and NH(3) deposition fluxes were 74.68-80.75 kgN ha(-1), which was equivalent to 162.4 and 175.5 kg ha(-1) of urea applied in 2006-2007. The N deposition fluxes were 13.91-40.38 and 5.33-22.73 kgN ha(-1) in peanut and rice growing periods, accounting for 8.18%-40.38% and 2.13%-23.06% of N fertilizer usages, respectively. NO(2) and NH(3) deposition were significant for the red soil farmland.

摘要

估算了2006—2007年期间大气氮(包括二氧化氮和氨)向中国东南部典型农业生态系统的干沉降。结果表明,二氧化氮和氨的干沉降速度分别为0.04—0.24厘米/秒和0.09—0.47厘米/秒。较高的值出现在非作物生长季节。大气中二氧化氮和氨的浓度分别为24.64—104.10微克氮/立方米和14.40—389.6微克氮/立方米。氨混合比的变化呈现明显的双峰。二氧化氮和氨的沉降通量为74.68—80.75千克氮/公顷,相当于2006—2007年施用的162.4和175.5千克/公顷尿素。花生和水稻生长季节的氮沉降通量分别为13.91—40.38和5.33—22.73千克氮/公顷,分别占氮肥用量的8.18%—40.38%和2.13%—23.06%。二氧化氮和氨的沉降对红壤农田具有重要意义。

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