• 文献检索
  • 文档翻译
  • 深度研究
  • 学术资讯
  • Suppr Zotero 插件Zotero 插件
  • 邀请有礼
  • 套餐&价格
  • 历史记录
应用&插件
Suppr Zotero 插件Zotero 插件浏览器插件Mac 客户端Windows 客户端微信小程序
定价
高级版会员购买积分包购买API积分包
服务
文献检索文档翻译深度研究API 文档MCP 服务
关于我们
关于 Suppr公司介绍联系我们用户协议隐私条款
关注我们

Suppr 超能文献

核心技术专利:CN118964589B侵权必究
粤ICP备2023148730 号-1Suppr @ 2026

文献检索

告别复杂PubMed语法,用中文像聊天一样搜索,搜遍4000万医学文献。AI智能推荐,让科研检索更轻松。

立即免费搜索

文件翻译

保留排版,准确专业,支持PDF/Word/PPT等文件格式,支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述,25分钟生成高质量综述,智能提取关键信息,辅助科研写作。

立即免费体验

带有电极的锯齿形石墨烯纳米带中边缘磁性的鲁棒性有限。

Limited robustness of edge magnetism in zigzag graphene nanoribbons with electrodes.

作者信息

Krompiewski S

机构信息

Institute of Molecular Physics, Polish Academy of Sciences, ul. M. Smoluchowskiego 17, 60179 Poznań, Poland.

出版信息

Nanotechnology. 2014 Nov 21;25(46):465201. doi: 10.1088/0957-4484/25/46/465201. Epub 2014 Oct 30.

DOI:10.1088/0957-4484/25/46/465201
PMID:25355693
Abstract

It is shown that apart from well-known factors, like temperature, substrate, and edge reconstruction effects, also the presence of external contacts is destructive for the formation of magnetic moments at the edges of graphene nanoribbons (GNRs). The edge magnetism gradually decreases when graphene/electrode interfaces become more and more transparent for electrons. In addition to the graphene/electrode coupling strength, the aspect ratio parameter, i.e. a width/length ratio of the GNR, is also crucial for the suppression of edge magnetism. The present theory uses a tight-binding method, based on the mean-field Hubbard Hamiltonian for π electrons, and the Green's function technique within the Landauer-Büttiker approach.

摘要

结果表明,除了温度、衬底和边缘重构效应等众所周知的因素外,外部接触的存在也会破坏石墨烯纳米带(GNRs)边缘磁矩的形成。当石墨烯/电极界面对于电子变得越来越透明时,边缘磁性会逐渐减弱。除了石墨烯/电极耦合强度外,纵横比参数,即GNR的宽度/长度比,对于抑制边缘磁性也至关重要。本理论采用紧束缚方法,基于π电子的平均场哈伯德哈密顿量,以及朗道尔-布蒂克尔方法中的格林函数技术。

相似文献

1
Limited robustness of edge magnetism in zigzag graphene nanoribbons with electrodes.带有电极的锯齿形石墨烯纳米带中边缘磁性的鲁棒性有限。
Nanotechnology. 2014 Nov 21;25(46):465201. doi: 10.1088/0957-4484/25/46/465201. Epub 2014 Oct 30.
2
A gate-induced switch in zigzag graphene nanoribbons and charging effects.锯齿型石墨烯纳米带中的栅极诱导开关和充电效应。
Nanotechnology. 2010 May 21;21(20):205306. doi: 10.1088/0957-4484/21/20/205306. Epub 2010 Apr 26.
3
Edge state magnetism of single layer graphene nanostructures.单层石墨烯纳米结构的边缘态磁性
J Chem Phys. 2008 Jun 28;128(24):244717. doi: 10.1063/1.2943678.
4
Effects of edge magnetism on the Kohn anomalies of zigzag graphene nanoribbons.边缘磁性对锯齿形石墨烯纳米带的科恩反常的影响。
Nanotechnology. 2016 Feb 12;27(6):065707. doi: 10.1088/0957-4484/27/6/065707. Epub 2016 Jan 14.
5
Electronic and magnetic properties of H-terminated graphene nanoribbons deposited on the topological insulator Sb2Te3.沉积在拓扑绝缘体Sb2Te3上的氢终止石墨烯纳米带的电子和磁性特性。
Sci Rep. 2016 Jul 11;6:29009. doi: 10.1038/srep29009.
6
A guide to the design of electronic properties of graphene nanoribbons.石墨烯纳米带电子性质设计指南。
Acc Chem Res. 2013 Oct 15;46(10):2319-28. doi: 10.1021/ar3001487.
7
Electronic transport through side-contacted graphene nanoribbons: effects of overlap, aspect ratio and orientation.通过侧边接触的石墨烯纳米带的电子输运:重叠、纵横比和取向的影响。
Nanotechnology. 2011 Nov 4;22(44):445201. doi: 10.1088/0957-4484/22/44/445201. Epub 2011 Oct 6.
8
Bandgap engineering of zigzag graphene nanoribbons by manipulating edge states via defective boundaries.通过在缺陷边界处操纵边缘态实现锯齿型石墨烯纳米带的能隙工程。
Nanotechnology. 2011 Oct 28;22(43):435702. doi: 10.1088/0957-4484/22/43/435702. Epub 2011 Oct 3.
9
Accurate prediction of the electronic properties of low-dimensional graphene derivatives using a screened hybrid density functional.使用屏蔽杂化密度泛函准确预测低维石墨烯衍生物的电子性质。
Acc Chem Res. 2011 Apr 19;44(4):269-79. doi: 10.1021/ar100137c. Epub 2011 Mar 9.
10
Magnetism in Nonplanar Zigzag Edge Termini of Graphene Nanoribbons.石墨烯纳米带非平面锯齿边缘末端的磁性。
Angew Chem Int Ed Engl. 2023 Jun 12;62(24):e202302534. doi: 10.1002/anie.202302534. Epub 2023 Apr 13.

引用本文的文献

1
Spin State Switching in Heptauthrene Nanostructure by Electric Field: Computational Study.电场诱导七并苯纳米结构中自旋态的转换:计算研究。
Int J Mol Sci. 2021 Dec 13;22(24):13364. doi: 10.3390/ijms222413364.