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利用电子全息术对银/氧化锌纳米天线进行电辐射映射

Electric radiation mapping of silver/zinc oxide nanoantennas by using electron holography.

作者信息

Sanchez J E, Mendoza-Santoyo F, Cantu-Valle J, Velazquez-Salazar J, José Yacaman M, González F J, Diaz de Leon R, Ponce A

机构信息

Department of Physics and Astronomy, University of Texas at San Antonio , San Antonio 78249, USA.

Coordinación para la Innovación y la Aplicación de la Ciencia y la Tecnología, Universidad Autónoma de San Luís Potosí , San Luis Potosí 78210, Mexico.

出版信息

J Appl Phys. 2015 Jan 21;117(3):034306. doi: 10.1063/1.4906102. Epub 2015 Jan 16.

Abstract

In this work, we report the fabrication of self-assembled zinc oxide nanorods grown on pentagonal faces of silver nanowires by using microwaves irradiation. The nanostructures resemble a hierarchal nanoantenna and were used to study the far and near field electrical metal-semiconductor behavior from the electrical radiation pattern resulting from the phase map reconstruction obtained using off-axis electron holography. As a comparison, we use electric numerical approximations methods for a finite number of ZnO nanorods on the Ag nanowires and show that the electric radiation intensities maps match closely the experimental results obtained with electron holography. The time evolution of the radiation pattern as generated from the nanostructure was recorded under radio frequency signal stimulation, in which the generated electrical source amplitude and frequency were varied from 0 to 5 V and from 1 to 10 MHz, respectively. The phase maps obtained from electron holography show the change in the distribution of the electric radiation pattern for individual nanoantennas. The mapping of this electrical behavior is of the utmost importance to gain a complete understanding for the metal-semiconductor (Ag/ZnO) heterojunction that will help to show the mechanism through which these receiving/transmitting structures behave at nanoscale level.

摘要

在这项工作中,我们报道了通过微波辐射在银纳米线的五边形面上生长自组装氧化锌纳米棒的制备方法。这些纳米结构类似于分层纳米天线,并被用于通过离轴电子全息术获得的相位图重建所产生的电辐射模式来研究远场和近场电金属-半导体行为。作为比较,我们对银纳米线上有限数量的氧化锌纳米棒使用电数值近似方法,并表明电辐射强度图与通过电子全息术获得的实验结果紧密匹配。在射频信号刺激下记录了由纳米结构产生的辐射模式的时间演化,其中产生的电源幅度和频率分别从0到5 V以及从1到10 MHz变化。从电子全息术获得的相位图显示了单个纳米天线电辐射模式分布的变化。这种电行为的映射对于全面理解金属-半导体(Ag/ZnO)异质结至关重要,这将有助于揭示这些接收/发射结构在纳米尺度上的行为机制。

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