Kumar Pratik, Bahl Shaila, Sahare P D, Kumar Surender, Singh Manveer
Medical Physics Unit, IRCH, AIIMS, New Delhi 110029, India
Medical Physics Unit, IRCH, AIIMS, New Delhi 110029, India.
Radiat Prot Dosimetry. 2015 Dec;167(4):453-60. doi: 10.1093/rpd/ncu371. Epub 2015 Feb 1.
This paper investigates the optically stimulated luminescence (OSL) response of BaFCl:Eu and K2Ca2(SO4)3:Eu phosphors for different doses and bleaching durations. The results have also been compared with the commercially available Landauer Al2O3:C (Luxel®) dosemeter. Nanocrystalline K2Ca2(SO4)3:Eu is known to be a sensitive thermoluminescent phosphor, but its OSL response is hardly reported. At first, pellets of nanocrystalline K2Ca2(SO4)3:Eu powder were prepared by adding Teflon as a binder. Their OSL signal was compared with that of the material in pure form, i.e. without adding the binder (in 100:1 ratio). It was observed that adding the binder does not appreciably affect the OSL intensity. On comparison with the commercially available Al2O3:C from Landauer, it was found that K2Ca2(SO4)3:Eu is around 15 times less sensitive than Al2O3:C. 'Homemade' BaFCl:Eu phosphor has also been studied. The intensity of BaFCl:Eu was ∼20 times more than the standard Al2O3:C dosemeter and ∼200 times more sensitive than K2Ca2(SO4)3:Eu in the dose range of 13-200 cGy. OSL dosemeters are believed to give luminescence signal even if they are read before, i.e. multiple reading may be possible under suitable conditions after single exposure. This was also checked for all the prepared dosemeters and it was found that Al2O3:C showed the least decrease of <2 %, followed by BaFCl:Eu of 15 % and K2Ca2(SO4)3:Eu with 20 %. Finally, Al2O3:C and BaFCl:Eu phosphors were also studied for their optical bleaching durations to which the respective signals get completely removed so that the phosphor can be re-used. It was observed that BaFCl:Eu is bleached faster and more easily than Al2O3:C.
本文研究了BaFCl:Eu和K2Ca2(SO4)3:Eu磷光体在不同剂量和漂白持续时间下的光激发发光(OSL)响应。研究结果还与市售的Landauer Al2O3:C(Luxel®)剂量计进行了比较。纳米晶K2Ca2(SO4)3:Eu是一种灵敏的热释光磷光体,但其OSL响应鲜有报道。首先,通过添加聚四氟乙烯作为粘结剂制备了纳米晶K2Ca2(SO4)3:Eu粉末颗粒。将它们的OSL信号与纯形式的材料(即不添加粘结剂,比例为100:1)的信号进行了比较。结果发现,添加粘结剂对OSL强度没有明显影响。与Landauer市售的Al2O3:C相比,发现K2Ca2(SO4)3:Eu的灵敏度比Al2O3:C低约15倍。还对“自制”的BaFCl:Eu磷光体进行了研究。在13 - 200 cGy的剂量范围内,BaFCl:Eu的强度比标准Al2O3:C剂量计高约20倍,比K2Ca2(SO4)3:Eu灵敏约200倍。人们认为,即使在单次曝光后在合适条件下多次读取,OSL剂量计也会发出发光信号。对所有制备的剂量计也进行了此项检查,结果发现Al2O3:C的降幅最小,小于2%,其次是BaFCl:Eu,降幅为15%,K2Ca2(SO4)3:Eu的降幅为20%。最后,还研究了Al2O3:C和BaFCl:Eu磷光体的光学漂白持续时间,即各自的信号完全消除,使磷光体能够重复使用所需的时间。结果发现,BaFCl:Eu比Al2O3:C漂白得更快、更容易。