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二阶颗粒状类固-液相转变的普遍性和临界性

Universality and criticality of a second-order granular solid-liquid-like phase transition.

作者信息

Castillo Gustavo, Mujica Nicolás, Soto Rodrigo

机构信息

Departamento de Física, Facultad de Ciencias Físicas y Matemáticas, Universidad de Chile, Avenida Blanco Encalada 2008, Santiago, Chile and Laboratoire de Physique Statistique, Ecole Normale Supérieure, UMR CNRS 8550, 24 Rue Lhomond, 75005 Paris, France.

Departamento de Física, Facultad de Ciencias Físicas y Matemáticas, Universidad de Chile, Avenida Blanco Encalada 2008, Santiago, Chile.

出版信息

Phys Rev E Stat Nonlin Soft Matter Phys. 2015 Jan;91(1):012141. doi: 10.1103/PhysRevE.91.012141. Epub 2015 Jan 26.

Abstract

We experimentally study the critical properties of the nonequilibrium solid-liquid-like transition that takes place in vibrated granular matter. The critical dynamics is characterized by the coupling of the density field with the bond-orientational order parameter Q(4), which measures the degree of local crystallization. Two setups are compared, which present the transition at different critical accelerations as a result of modifying the energy dissipation parameters. In both setups five independent critical exponents are measured, associated to different properties of Q(4): the correlation length, relaxation time, vanishing wavenumber limit (static susceptibility), the hydrodynamic regime of the pair correlation function, and the amplitude of the order parameter. The respective critical exponents agree in both setups and are given by ν(⊥)=1,ν(∥)=2,γ=1,η≈0.6-0.67, and β=1/2, whereas the dynamical critical exponent is z=ν(∥)/ν(⊥)=2. The agreement on five exponents is an exigent test for the universality of the transition. Thus, while dissipation is strictly necessary to form the crystal, the path the system undergoes toward the phase separation is part of a well-defined universality class. In fact, the local order shows critical properties while density does not. Being the later conserved, the appropriate model that couples both is model C in the Hohenberg and Halperin classification. The measured exponents are in accord with the nonequilibrium extension to model C if we assume that α, the exponent associated in equilibrium to the specific heat divergence but with no counterpart in this nonequilibrium experiment, vanishes.

摘要

我们通过实验研究了振动颗粒物质中发生的非平衡类固 - 液转变的临界性质。临界动力学由密度场与键取向序参量(Q(4))的耦合来表征,(Q(4))用于衡量局部结晶程度。比较了两种实验装置,由于修改了能量耗散参数,它们在不同的临界加速度下呈现出转变。在这两种装置中,测量了五个独立的临界指数,它们与(Q(4))的不同性质相关:关联长度、弛豫时间、零波数极限(静态磁化率)、对关联函数的流体动力学区域以及序参量的振幅。两种装置中的相应临界指数一致,分别为(\nu(\perp)=1),(\nu(\parallel)=2),(\gamma = 1),(\eta\approx0.6 - 0.67),以及(\beta = 1/2),而动力学临界指数为(z = \nu(\parallel)/\nu(\perp)=2)。五个指数的一致性是对该转变普遍性的严格检验。因此,虽然形成晶体严格需要耗散,但系统走向相分离的路径是一个定义明确的普适类的一部分。实际上,局部有序呈现出临界性质,而密度则不然。由于密度是守恒的,将两者耦合的合适模型是霍恩伯格和哈珀林分类中的模型C。如果我们假设在平衡态中与比热发散相关但在此非平衡实验中无对应项的指数(\alpha)为零,那么测量得到的指数与模型C的非平衡扩展是一致的。

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