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一种用于环境分析的高效高纯锗符合系统。

A high-efficiency HPGe coincidence system for environmental analysis.

作者信息

Britton R, Davies A V, Burnett J L, Jackson M J

机构信息

AWE, Aldermaston, Reading, Berkshire, RG7 4PR, UK; University of Surrey, Guildford, GU2 7XH, UK.

AWE, Aldermaston, Reading, Berkshire, RG7 4PR, UK.

出版信息

J Environ Radioact. 2015 Aug;146:1-5. doi: 10.1016/j.jenvrad.2015.03.033. Epub 2015 Apr 11.

Abstract

The Comprehensive Nuclear-Test-Ban Treaty (CTBT) is supported by a network of certified laboratories which must meet certain sensitivity requirements for CTBT relevant radionuclides. At the UK CTBT Radionuclide Laboratory (GBL15), a high-efficiency, dual-detector gamma spectroscopy system has been developed to improve the sensitivity of measurements for treaty compliance, greatly reducing the time required for each sample. Utilising list-mode acquisition, each sample can be counted once, and processed multiple times to further improve sensitivity. For the 8 key radionuclides considered, Minimum Detectable Activities (MDA's) were improved by up to 37% in standard mode (when compared to a typical CTBT detector system), with the acquisition time required to achieve the CTBT sensitivity requirements reduced from 6 days to only 3. When utilising the system in coincidence mode, the MDA for (60) Co in a high-activity source was improved by a factor of 34 when compared to a standard CTBT detector, and a factor of 17 when compared to the dual-detector system operating in standard mode. These MDA improvements will allow the accurate and timely quantification of radionuclides that decay via both singular and cascade γ emission, greatly enhancing the effectiveness of CTBT laboratories.

摘要

《全面禁止核试验条约》(CTBT)得到了一个经过认证的实验室网络的支持,这些实验室必须满足对与CTBT相关的放射性核素的某些灵敏度要求。在英国CTBT放射性核素实验室(GBL15),已经开发了一种高效的双探测器伽马能谱系统,以提高用于条约合规性测量的灵敏度,大大减少每个样品所需的时间。利用列表模式采集,每个样品可以计数一次,并进行多次处理以进一步提高灵敏度。对于所考虑的8种关键放射性核素,在标准模式下(与典型的CTBT探测器系统相比),最低探测活度(MDA)提高了37%,达到CTBT灵敏度要求所需的采集时间从6天减少到仅3天。当在符合模式下使用该系统时,与标准CTBT探测器相比,高活度源中(60)Co的MDA提高了34倍,与在标准模式下运行的双探测器系统相比提高了17倍。这些MDA的提高将允许对通过单能和级联γ发射衰变的放射性核素进行准确和及时的定量,大大提高CTBT实验室的效能。

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