†Mechanical Engineering Department, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, United States.
‡IBM T.J. Watson Research Center, 1101 Kitchawan Road, Yorktown Heights, New York 10598, United States.
Nano Lett. 2015 May 13;15(5):3172-80. doi: 10.1021/acs.nanolett.5b01191. Epub 2015 Apr 27.
Hexagonal boron nitride (hBN) is a natural hyperbolic material, which can also accommodate highly dispersive surface phonon-polariton modes. In this paper, we examine theoretically the mid-infrared optical properties of graphene-hBN heterostructures derived from their coupled plasmon-phonon modes. We find that the graphene plasmon couples differently with the phonons of the two Reststrahlen bands, owing to their different hyperbolicity. This also leads to distinctively different interaction between an external quantum emitter and the plasmon-phonon modes in the two bands, leading to substantial modification of its spectrum. The coupling to graphene plasmons allows for additional gate tunability in the Purcell factor and narrow dips in its emission spectra.
六方氮化硼(hBN)是一种天然的双曲材料,也能容纳高度色散的表面声子极化激元模式。在本文中,我们从耦合等离子体-声子模式的角度理论上研究了石墨烯- hBN 异质结构的中红外光学性质。我们发现,由于双曲性不同,石墨烯等离子体与两个瑞利带的声子的耦合方式也不同。这也导致了外部量子发射器与两个带中的等离子体-声子模式之间的相互作用明显不同,从而导致其光谱发生实质性的改变。与石墨烯等离子体的耦合使得在普塞尔因子中增加了额外的栅极可调性,并在其发射光谱中产生了狭窄的凹陷。