Departamento de Química Inorgánica, Cristalografía y Mineralogía, Facultad de Ciencias, Universidad de Málaga, Campus de Teatinos, 29071 Málaga, Spain.
Departamento de Química Inorgánica, Cristalografía y Mineralogía, Facultad de Ciencias, Universidad de Málaga, Campus de Teatinos, 29071 Málaga, Spain.
J Hazard Mater. 2015 Oct 15;296:112-119. doi: 10.1016/j.jhazmat.2015.04.021. Epub 2015 Apr 9.
Ni2P and CoP catalysts (5 wt.% of metal) supported on a commercial SiO2 were tested in the gas phase catalytic hydrodechlorination (HDCl) of mono (chlorobenzene-ClB) and polychlorobenzenes (PCBs) (1,2- dichlorobenzene (1,2-DClB), 1,3-dichlorobenzene (1,3-DClB), 1,4-dichlorobenzene (1,4-DClB), and 1,2,4-trichlorobenzene (1,2,4-TClB)) at atmospheric pressure. It was investigated how the number and position of chlorine atoms in the molecule influence the HDCl activity. The prepared catalysts were characterized by X-ray diffraction (XRD), CO chemisorption, N2 adsorption-desorption at -196°C, and X-ray photoelectron spectroscopy (XPS). Characterization results indicated better active phase dispersion and greater amount of P on the Ni2P catalyst surface. Catalytic results showed that the Ni2P was more active and stable in this type of reactions. The hydrodechlorination activity decreased by increasing the number of chlorine atoms in the molecule and chlorine substituents in close proximity. The observed trend in the HDCl activity was: ClB>1,4-DClB>1,3-DClB>1,2-DClB>1,2,4-TClB. The exception was the catalytic response after 24h on stream observed for the Ni2P in the HDCl reaction of 1,2,4-TClB, which was equal to that observed for the 1,4-DClB molecule, and also yielding benzene as the main reaction product.
在常压下,负载在商业 SiO2 上的 Ni2P 和 CoP 催化剂(金属含量为 5wt.%)被用于气相催化脱氯(HDCl)单氯苯(ClB)和多氯苯(PCBs)(1,2-二氯苯(1,2-DClB)、1,3-二氯苯(1,3-DClB)、1,4-二氯苯(1,4-DClB)和 1,2,4-三氯苯(1,2,4-TClB))。研究了分子中氯原子的数量和位置如何影响 HDCl 活性。通过 X 射线衍射(XRD)、CO 化学吸附、-196°C 下的 N2 吸附-脱附和 X 射线光电子能谱(XPS)对制备的催化剂进行了表征。表征结果表明 Ni2P 催化剂表面的活性相分散性更好,磷含量更高。催化结果表明,Ni2P 在这类反应中更活跃、更稳定。随着分子中氯原子数量的增加和氯取代基的接近,脱氯活性降低。HDCl 活性的观察趋势为:ClB>1,4-DClB>1,3-DClB>1,2-DClB>1,2,4-TClB。例外的是在 Ni2P 催化 1,2,4-TClB 的 HDCl 反应中,在 24 小时连续运行后的催化响应与 1,4-DClB 分子相同,并且苯也是主要的反应产物。