Häfele Verena, Trügler Andreas, Hohenester Ulrich, Hohenau Andreas, Leitner Alfred, Krenn Joachim R
Opt Express. 2015 Apr 20;23(8):10293-300. doi: 10.1364/OE.23.010293.
We experimentally investigate the local refractive index sensitivity of plasmonic gold nanodisks by applying small polymer dots to selected disk sites by means of two-step lithography. Measured sensitivity profiles obtained from tracking the polymer-induced spectral shift of the plasmon modes are in excellent agreement with numerical simulation of both spectral sensitivity and the electric near field of the nanodisks. Based on the nanodisk sensitivity profile we tailor a sensitive and spatially uniform plasmonic sensor by capping the disk with a dielectric layer, thus restricting analyte access to the disk rim.
我们通过两步光刻法将小聚合物点应用于选定的金纳米盘位点,对等离子体金纳米盘的局部折射率灵敏度进行了实验研究。通过跟踪聚合物诱导的等离子体模式光谱位移获得的测量灵敏度曲线,与纳米盘光谱灵敏度和近场电场的数值模拟结果高度吻合。基于纳米盘的灵敏度曲线,我们通过在纳米盘上覆盖一层介电层来定制一种灵敏且空间均匀的等离子体传感器,从而限制分析物进入盘边缘。