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单光子与双光子对动力学隧穿的控制:非规则弗洛凯态的影响

One Versus Two Photon Control of Dynamical Tunneling: Influence of the Irregular Floquet States.

作者信息

Shukla Archana, Keshavamurthy Srihari

机构信息

Department of Chemistry, Indian Institute of Technology , Kanpur, Uttar Pradesh 208 016, India.

出版信息

J Phys Chem B. 2015 Aug 27;119(34):11326-35. doi: 10.1021/acs.jpcb.5b03299. Epub 2015 Jun 19.

Abstract

A useful approach to control quantum processes involves driving systems with two colored laser fields and varying the relative phase between the fields to control the quantum interferences. A particularly interesting class of bichromatic control schemes involves the so-called M versus N-photon control that results in laser-induced symmetry breaking and leads to directed transport; however, recent studies have shown that the mechanism of laser-induced symmetry breaking has a common classical and quantum origin. In this context, a relevant question is the extent to which such a detailed classical-quantum correspondence holds if the process to be controlled involves quantum tunneling. In this work, we address this issue in terms of controlling dynamical tunneling between field-induced islands of stability in the classical phase space of a model system, a periodically driven pendulum. This is also a paradigmatic model for Hamiltonian ratchets wherein the islands of stability, that is, nonlinear resonances, play a crucial role in the observed directed transport. We compute an appropriate control landscape for the process and show that despite breaking the relevant symmetries, there exist regions in the control landscape where the control fails. The lack of control can be understood in terms of the phase-space nature of the quantum Floquet states that participate in the dynamics of the initial wavepacket. We argue that robust regions of no control arise due to the phenomenon of chaos-assisted tunneling and comment on the possible influence of such regions on the directed transport in the model system.

摘要

一种控制量子过程的有效方法是用两个有色激光场驱动系统,并改变场之间的相对相位来控制量子干涉。一类特别有趣的双色控制方案涉及所谓的M对N光子控制,这种控制会导致激光诱导的对称性破缺并导致定向输运;然而,最近的研究表明,激光诱导对称性破缺的机制有一个共同的经典和量子起源。在这种情况下,一个相关的问题是,如果要控制的过程涉及量子隧穿,这种详细的经典-量子对应在多大程度上成立。在这项工作中,我们通过控制一个模型系统(一个周期性驱动的摆)经典相空间中场诱导的稳定岛之间的动态隧穿来解决这个问题。这也是哈密顿棘轮的一个典型模型,其中稳定岛,即非线性共振,在观察到的定向输运中起着关键作用。我们计算了该过程的适当控制态势,并表明尽管打破了相关对称性,但在控制态势中仍存在控制失败的区域。缺乏控制可以根据参与初始波包动力学的量子弗洛凯态的相空间性质来理解。我们认为,由于混沌辅助隧穿现象,会出现无控制的稳健区域,并评论了这些区域对模型系统中定向输运的可能影响。

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