Environ Sci Technol. 2015 Jul 7;49(13):8139-46. doi: 10.1021/es5063055.
Atmospheric methane (CH4) was measured using a mobile laboratory to quantify fugitive CH4 emissions from Oil and Natural Gas (ONG) operations in the Barnett Shale area. During this Barnett Coordinated Campaign we sampled more than 152 facilities, including well pads, compressor stations, gas processing plants, and landfills. Emission rates from several ONG facilities and landfills were estimated using an Inverse Gaussian Dispersion Model and the Environmental Protection Agency (EPA) Model AERMOD. Model results show that well pads emissions rates had a fat-tailed distribution, with the emissions linearly correlated with gas production. Using this correlation, we estimated a total well pad emission rate of 1.5 × 10(5) kg/h in the Barnett Shale area. It was found that CH4 emissions from compressor stations and gas processing plants were substantially higher, with some "super emitters" having emission rates up to 3447 kg/h, more then 36,000-fold higher than reported by the Environmental Protection Agency (EPA) Greenhouse Gas Reporting Program (GHGRP). Landfills are also a significant source of CH4 in the Barnett Shale area, and they should be accounted for in the regional budget of CH4.
采用移动实验室对大气甲烷(CH4)进行了测量,以量化 Barnett 页岩地区石油和天然气(ONG)作业中的逸散 CH4 排放。在此次 Barnett 协调行动期间,我们对超过 152 个设施进行了采样,包括井场、压缩机站、天然气处理厂和垃圾填埋场。使用反高斯扩散模型和美国环保署(EPA)的 AERMOD 模型估算了一些 ONG 设施和垃圾填埋场的排放速率。模型结果表明,井场排放速率呈长尾分布,排放量与天然气产量呈线性相关。利用这种相关性,我们估算出 Barnett 页岩地区的总井场排放量为 1.5×10(5)kg/h。研究发现,压缩机站和天然气处理厂的 CH4 排放量要高得多,一些“超级排放源”的排放速率高达 3447kg/h,比美国环保署(EPA)温室气体报告计划(GHGRP)报告的数值高出 36000 多倍。垃圾填埋场也是 Barnett 页岩地区 CH4 的重要来源,应将其纳入 CH4 的区域预算中。