College of Architecture and Environment, Sichuan University, Chengdu 610065, China; MOE Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, Tianjin 300071, China.
College of Architecture and Environment, Sichuan University, Chengdu 610065, China.
Sci Total Environ. 2015 Dec 1;536:288-294. doi: 10.1016/j.scitotenv.2015.07.057. Epub 2015 Jul 25.
A total of 688 samples, including 520 food samples belonging to 29 food types in 10 groups, 63 drinking water, and 105 indoor dust samples were collected during May to November in 2014 in Chengdu and Tianjin (only dust samples in Tianjin), China to investigate the perchlorate levels in these samples and to estimate the related exposure to Chinese people. Significant difference in indoor dust perchlorate levels was found between Chengdu and Tianjin, with the concentrations ranging from 0.11 to 38.8 mg/kg in Chengdu, and from 0.72 to 119 mg/kg in Tianjin. The mean perchlorate levels in 10 groups of food samples were in the order of vegetables>wheaten flour≈egg, and wheaten flour>milk>sea food>livestock meats≈poultry≈freshwater fish>fruits>steamed rice, while no statistical difference in perchlorate levels was found between egg and milk. Exposure evaluation indicated that indoor dust contributed little (less than 5%) to the total daily perchlorate intake, and food consumption was the primary perchlorate exposure route for Chengdu people, followed by drinking water. Based on the median perchlorate levels obtained in this study, the daily perchlorate intake was below the reference does suggested by the US EPA.
共采集 688 个样本,包括 2014 年 5 月至 11 月在中国成都和天津(仅天津采集室内灰尘样本)采集的 10 组 29 种食物样本 520 个,饮用水样本 63 个,室内灰尘样本 105 个,用以调查这些样本中的高氯酸盐含量,并评估中国人的相关暴露情况。成都和天津的室内灰尘中高氯酸盐含量存在显著差异,浓度范围分别为 0.11 至 38.8 毫克/千克和 0.72 至 119 毫克/千克。10 组食物样本的高氯酸盐平均含量依次为蔬菜>小麦粉≈鸡蛋,以及小麦粉>牛奶>海鲜>畜肉≈禽肉>淡水鱼>水果>米饭,而鸡蛋和牛奶中的高氯酸盐含量没有统计学差异。暴露评估表明,室内灰尘对总日高氯酸盐摄入量的贡献较小(<5%),食物消费是成都人高氯酸盐暴露的主要途径,其次是饮用水。基于本研究中获得的高氯酸盐中位数水平,每日高氯酸盐摄入量低于美国环保署建议的参考剂量。