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固体环境样品中低γ能放射性核素铅测定的自吸收校正快速程序。

Fast procedure for self-absorption correction for low γ energy radionuclide Pb determination in solid environmental samples.

作者信息

Długosz-Lisiecka Magdalena, Bem Henryk

机构信息

Technical University of Lodz, Institute of Applied Radiation Chemistry, Zeromskiego Street 116, 90-924 Lodz, Poland.

出版信息

J Radioanal Nucl Chem. 2013;298(1):495-499. doi: 10.1007/s10967-012-2404-8. Epub 2013 Jan 24.

DOI:10.1007/s10967-012-2404-8
PMID:26224939
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC4514590/
Abstract

Low-energy X and γ radiations (for example of Pb:  = 46.5 keV) are effectively self-absorbed even in thin environmental samples, including air filters with captured dust or contaminated soil, as well as in bottom sediment matrixes with limited quantities of the samples. In this paper, a simple method for the direct analysis of Pb ( = 22.3 years) by gamma-ray spectrometry in environmental samples with self-absorption correction is described. The method is based on the comparison of two γ peak activities coming from other natural radionuclides, usually present in environmental samples. We have analyzed the dependence of the self-absorption correction factor for the Pb activity on the activity ratios of 911 and 209 keV peaks and 609 and 295 keV peaks coming from nuclides of U or Th rows, present in typical environmental samples.

摘要

低能X射线和γ射线辐射(例如铅的辐射:能量为46.5 keV)即使在稀薄的环境样品中也会被有效自吸收,这些样品包括带有捕获灰尘的空气过滤器或受污染土壤,以及样品量有限的底部沉积物基质。本文描述了一种通过γ射线光谱法对环境样品中的铅(半衰期为22.3年)进行直接分析并进行自吸收校正的简单方法。该方法基于对环境样品中通常存在的其他天然放射性核素产生的两个γ峰活度的比较。我们分析了典型环境样品中铀系或钍系核素产生的911和209 keV峰以及609和295 keV峰的活度比与铅活度自吸收校正因子之间的关系。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ac8a/4514590/a6aba3e22dd3/10967_2012_2404_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ac8a/4514590/a6aba3e22dd3/10967_2012_2404_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ac8a/4514590/a6aba3e22dd3/10967_2012_2404_Fig1_HTML.jpg

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本文引用的文献

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Determination of the mean aerosol residence times in the atmosphere and additional Po input on the base of simultaneous determination of Be, Na, Pb, Bi and Po in urban air.基于对城市空气中铍、钠、铅、铋和钋的同步测定来确定大气中气溶胶的平均停留时间以及额外的钋输入量。
J Radioanal Nucl Chem. 2012;293(1):135-140. doi: 10.1007/s10967-012-1690-5. Epub 2012 Feb 29.
2
A simplified gamma-ray self-attenuation correction in bulk samples.
Appl Radiat Isot. 2008 Mar;66(3):407-13. doi: 10.1016/j.apradiso.2007.10.007. Epub 2007 Dec 3.
3
Determination of self-absorption corrections for gamma analysis of environmental samples: comparing gamma-absorption curves and spiked matrix-matched samples.环境样品γ分析中自吸收校正的测定:比较γ吸收曲线和加标基质匹配样品
Appl Radiat Isot. 2004 Feb-Apr;60(2-4):571-7. doi: 10.1016/j.apradiso.2003.11.081.
4
Use of HPGe gamma-ray spectrometry to assess the isotopic compositiion of uranium in soils.使用高纯锗γ射线能谱法评估土壤中铀的同位素组成。
J Environ Radioact. 2003;64(2-3):195-203. doi: 10.1016/s0265-931x(02)00049-8.
5
A simplified technique to determine the self-absorption correction for sediment samples.一种用于确定沉积物样品自吸收校正的简化技术。
Appl Radiat Isot. 2002 Dec;57(6):915-8. doi: 10.1016/s0969-8043(02)00169-0.
6
Monte Carlo simulation of the self-absorption corrections for natural samples in gamma-ray spectrometry.γ射线能谱法中天然样品自吸收校正的蒙特卡罗模拟
Appl Radiat Isot. 2002 Dec;57(6):893-8. doi: 10.1016/s0969-8043(02)00220-8.
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Corrections for self-attenuation in gamma-ray spectrometry of bulk samples.块状样品γ射线能谱分析中自吸收的校正
Appl Radiat Isot. 2001 May;54(5):777-83. doi: 10.1016/s0969-8043(00)00319-5.