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加标放射性氙气的空气。

Radioxenon spiked air.

作者信息

Watrous Matthew G, Delmore James E, Hague Robert K, Houghton Tracy P, Jenson Douglas D, Mann Nick R

机构信息

Idaho National Laboratory, 2525 N. Fremont Avenue, Idaho Falls, ID 83415, USA.

Idaho National Laboratory, 2525 N. Fremont Avenue, Idaho Falls, ID 83415, USA.

出版信息

J Environ Radioact. 2015 Dec;150:126-31. doi: 10.1016/j.jenvrad.2015.08.005. Epub 2015 Aug 27.

Abstract

Four of the radioactive xenon isotopes ((131m)Xe, (133m)Xe, (133)Xe and (135)Xe) with half-lives ranging from 9 h to 12 days are produced from nuclear fission and can be detected from days to weeks following their production and release. Being inert gases, they are readily transported through the atmosphere. Sources for release of radioactive xenon isotopes include operating nuclear reactors via leaks in fuel rods, medical isotope production facilities, and nuclear weapons' detonations. They are not normally released from fuel reprocessing due to the short half-lives. The Comprehensive Nuclear-Test-Ban Treaty has led to creation of the International Monitoring System. The International Monitoring System, when fully implemented, will consist of one component with 40 stations monitoring radioactive xenon around the globe. Monitoring these radioactive xenon isotopes is important to the Comprehensive Nuclear-Test-Ban Treaty in determining whether a seismically detected event is or is not a nuclear detonation. A variety of radioactive xenon quality control check standards, quantitatively spiked into various gas matrices, could be used to demonstrate that these stations are operating on the same basis in order to bolster defensibility of data across the International Monitoring System. This paper focuses on Idaho National Laboratory's capability to produce three of the xenon isotopes in pure form and the use of the four xenon isotopes in various combinations to produce radioactive xenon spiked air samples that could be subsequently distributed to participating facilities.

摘要

四种放射性氙同位素((131m)Xe、(133m)Xe、(133)Xe和(135)Xe)的半衰期从9小时到12天不等,由核裂变产生,在其产生和释放后的数天到数周内都能被检测到。作为惰性气体,它们很容易在大气中传输。放射性氙同位素的释放源包括运行中的核反应堆(通过燃料棒泄漏)、医用同位素生产设施以及核武器爆炸。由于半衰期短,它们通常不会从燃料后处理过程中释放出来。《全面禁止核试验条约》促成了国际监测系统的建立。国际监测系统全面实施后,将包括一个由40个监测站组成的部分,用于监测全球范围内的放射性氙。监测这些放射性氙同位素对于《全面禁止核试验条约》确定地震探测到的事件是否为核爆炸非常重要。可以使用多种定量添加到各种气体基质中的放射性氙质量控制检查标准,来证明这些监测站在相同的基础上运行,以加强整个国际监测系统数据的可信度。本文重点介绍爱达荷国家实验室以纯形式生产三种氙同位素的能力,以及使用四种氙同位素的各种组合来生产放射性氙加标空气样本,这些样本随后可分发给参与的设施。

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