Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, UK.
Nature. 2015 Sep 10;525(7568):222-5. doi: 10.1038/nature14868. Epub 2015 Aug 31.
Resonance fluorescence arises from the interaction of an optical field with a two-level system, and has played a fundamental role in the development of quantum optics and its applications. Despite its conceptual simplicity, it entails a wide range of intriguing phenomena, such as the Mollow-triplet emission spectrum, photon antibunching and coherent photon emission. One fundamental aspect of resonance fluorescence--squeezing in the form of reduced quantum fluctuations in the single photon stream from an atom in free space--was predicted more than 30 years ago. However, the requirement to operate in the weak excitation regime, together with the combination of modest oscillator strength of atoms and low collection efficiencies, has continued to necessitate stringent experimental conditions for the observation of squeezing with atoms. Attempts to circumvent these issues had to sacrifice antibunching, owing to either stimulated forward scattering from atomic ensembles or multi-photon transitions inside optical cavities. Here, we use an artificial atom with a large optical dipole enabling 100-fold improvement of the photon detection rate over the natural atom counterpart and reach the necessary conditions for the observation of quadrature squeezing in single resonance-fluorescence photons. By implementing phase-dependent homodyne intensity-correlation detection, we demonstrate that the electric field quadrature variance of resonance fluorescence is three per cent below the fundamental limit set by vacuum fluctuations, while the photon statistics remain antibunched. The presence of squeezing and antibunching simultaneously is a fully non-classical outcome of the wave-particle duality of photons.
共振荧光源于光场与二能级系统的相互作用,在量子光学及其应用的发展中发挥了基础作用。尽管其概念简单,但它涉及到广泛的有趣现象,如 Mollow 三重态发射光谱、光子反聚束和相干光子发射。共振荧光的一个基本方面——在自由空间中原子的单光子流中减少量子涨落的形式的压缩——在 30 多年前就已经被预测到了。然而,为了在弱激发条件下工作,以及原子的振子强度适中且收集效率低,这就需要严格的实验条件来观察原子的压缩。为了规避这些问题,由于原子系综中的受激前向散射或光学腔中的多光子跃迁,不得不牺牲反聚束。在这里,我们使用一个具有大光学偶极子的人工原子,使光子探测率比天然原子提高了 100 倍,并达到了观察单共振荧光光子中正交压缩的必要条件。通过实施相位相关的同相强度相关检测,我们证明了共振荧光的电场正交方差比真空涨落设定的基本极限低 3%,而光子统计仍然反聚束。压缩和反聚束同时存在是光子波粒二象性的完全非经典结果。