Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, United Kingdom.
Phys Rev Lett. 2012 Mar 2;108(9):093602. doi: 10.1103/PhysRevLett.108.093602. Epub 2012 Feb 28.
The observation of quantum-dot resonance fluorescence enabled a new solid-state approach to generating single photons with a bandwidth approaching the natural linewidth of a quantum-dot transition. Here, we operate in the small Rabi frequency limit of resonance fluorescence--the Heitler regime--to generate subnatural linewidth and high-coherence quantum light from a single quantum dot. The measured single-photon coherence is 30 times longer than the lifetime of the quantum-dot transition, and the single photons exhibit a linewidth which is inherited from the excitation laser. In contrast, intensity-correlation measurements reveal that this photon source maintains a high degree of antibunching behavior on the order of the transition lifetime with vanishing two-photon scattering probability. Generating decoherence-free phase-locked single photons from multiple quantum systems will be feasible with our approach.
量子点共振荧光的观测使人们能够采用一种新的固态方法来产生带宽接近量子点跃迁自然线宽的单光子。在这里,我们在共振荧光的小拉比频率极限(海特勒 regime)下工作,从而能够从单个量子点产生亚自然线宽和高相干度的量子光。所测量的单光子相干性比量子点跃迁的寿命长 30 倍,并且单光子的线宽继承自激发激光。相比之下,强度相关测量显示,这种光子源在与跃迁寿命相当的时间尺度上保持着高度的反聚束行为,并且双光子散射概率趋近于零。通过我们的方法,从多个量子系统中产生无退相干锁定的单光子将成为可能。