Xu Wei, Huang Jun-Jun, Shao Bin-Hao, Xu Xing-Jie, Jiang Ren-Wang, Yuan Mu
Pharmaceutical Research Center, Guangzhou Medical University, 195# Dongfengxi Road, Guangzhou 510182, China.
School of Pharmaceutical Sciences, Jinan University, Guangzhou 510632, China.
Molecules. 2015 Oct 30;20(11):19674-89. doi: 10.3390/molecules201119651.
Indole-arylpiperazine derivatives have exhibited good selectivity for the α1A-adrenoceptor, but the structure-activity-binding mechanism relationship remains unclear. In the current study, three compounds (1, 2 and 3) were investigated through single-crystal X-ray diffraction analysis, density functional theory (DFT) calculations and molecular docking using a homology model of the α1A receptor. Compounds 1 and 3 form H-bonds networks to stabilize their three-dimensional structures, while C-H···π interactions play a significant role in the packing of 2. Based on DFT-optimized conformations, the HOMO-LUMO energy gaps and molecular electrostatic potential (MEP) were theoretically calculated at the B3LYP/6-311G (d, p) level of theory. Chemical reactivity increases in the order of 3 < 2 < 1, and the maximum positive region of the MEP maps is mainly localized over the NH group. The binding mechanisms of ligand-α1A-adrenoceptor complexes were illustrated by molecular docking. Binding to Gln177 of the second extracellular loop region via hydrogen bonds is likely to be essential for α1A-selective antagonists. The present work sheds light on the studies of structure-activity-binding mechanism and aids in the design of α1A antagonists with high selectivity.
吲哚 - 芳基哌嗪衍生物对α1A - 肾上腺素能受体表现出良好的选择性,但构效关系与结合机制仍不清楚。在本研究中,通过单晶X射线衍射分析、密度泛函理论(DFT)计算以及使用α1A受体同源模型的分子对接,对三种化合物(1、2和3)进行了研究。化合物1和3形成氢键网络以稳定其三维结构,而C - H···π相互作用在化合物2的堆积中起重要作用。基于DFT优化的构象,在B3LYP/6 - 311G(d, p)理论水平上理论计算了最高占据分子轨道(HOMO)-最低未占据分子轨道(LUMO)能隙和分子静电势(MEP)。化学反应性按3 < 2 < 1的顺序增加,MEP图的最大正区域主要位于NH基团上。通过分子对接阐明了配体 - α1A - 肾上腺素能受体复合物的结合机制。通过氢键与第二个细胞外环区域的Gln177结合可能是α1A选择性拮抗剂的关键。本研究为构效关系与结合机制的研究提供了线索,并有助于设计具有高选择性的α1A拮抗剂。