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大坝建设后沉积物中重金属积累的空间分布。

Spatial distribution of heavy metal accumulation in the sediments after dam construction.

作者信息

Shim Moo Joon, Yang Yun Mo, Oh Da Yeon, Lee Soo Hyung, Yoon Yi Yong

机构信息

Geum River Environment Research Center, National Institute of Environmental Research, Okcheon, South Korea, 373-804.

Department of Environmental Engineering, Catholic Kwandong University, Gangneung, South Korea, 210-701.

出版信息

Environ Monit Assess. 2015 Dec;187(12):733. doi: 10.1007/s10661-015-4967-7. Epub 2015 Nov 9.

Abstract

The sedimentary environment has been modified in the Geum River where an estuary dam and midstream dams were constructed. Furthermore, the Geum River tributaries deliver contaminants from the wastewater of an industrial complex. However, the influence of tributaries and dams on sedimentary metal deposition has not been extensively studied. The objectives of this study are to assess metal accumulation and to investigate the source of the metals. Sediments were collected in the main channel and two tributaries on October 2013. Abnormal accumulations of fine sediments were not observed above the midstream dams. Chromium, Ni, and Zn showed higher concentrations in above the midstream dam, but their concentrations were not related to grain size. Cadmium, Cu, Pb, and Hg were much higher upstream from the first midstream dam and came from one of the major tributaries. Arsenic was the only element found at higher concentrations downstream from the last midstream dam and was likely sourced from abandoned mines and/or agricultural activity. The pollution indexes indicated deposition of all metals, except Cr and Ni, may have been affected by anthropogenic activity. With respect to long-term accumulation of the metals, accumulation of Pb, Zn, and Cu by anthropogenic input largely increased, implying accumulation of these metals has continued due to anthropogenic activity since the estuary dam was constructed. Our results suggest that changes in river flow caused by the estuary dam and anthropogenic input from tributaries sources increased the accumulation of heavy metals (e.g., Pb, Zn, Cu, and As).

摘要

锦江修建了河口大坝和中游大坝,其沉积环境已被改变。此外,锦江的支流还输送来自工业园区废水的污染物。然而,支流和大坝对沉积金属沉积的影响尚未得到广泛研究。本研究的目的是评估金属积累情况并调查金属的来源。2013年10月在主河道和两条支流采集了沉积物。在中游大坝上方未观察到细颗粒沉积物的异常堆积。铬、镍和锌在中游大坝上方浓度较高,但它们的浓度与粒度无关。镉、铜、铅和汞在第一个中游大坝上游要高得多,且来自一条主要支流。砷是在最后一个中游大坝下游发现浓度较高的唯一元素,可能来自废弃矿山和/或农业活动。污染指数表明,除铬和镍外,所有金属的沉积可能都受到了人为活动的影响。关于金属的长期积累,人为输入导致的铅、锌和铜的积累大幅增加,这意味着自河口大坝建成以来,由于人为活动,这些金属的积累一直在持续。我们的结果表明,河口大坝导致的河流流量变化以及支流来源的人为输入增加了重金属(如铅、锌、铜和砷)的积累。

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