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电流诱导力:一种在分子结中诱导负微分电阻和电流开关效应的新机制。

Current-induced forces: a new mechanism to induce negative differential resistance and current-switching effect in molecular junctions.

作者信息

Gu Lei, Fu Hua-Hua

机构信息

College of Physics and Wuhan National High Magnetic field center, Huazhong University of Science and Technology, Wuhan 430074, People's Republic of China.

出版信息

Nanotechnology. 2015 Dec 4;26(48):485703. doi: 10.1088/0957-4484/26/48/485703. Epub 2015 Nov 12.

Abstract

Current-induced forces can excite molecules, polymers and other low-dimensional materials, which in turn leads to an effective gate voltage through Holstein interaction. Here, by taking a short asymmetric DNA junction as an example, and using the Langevin approach, we find that when suppression of charge transport by the effective gate voltage surpasses the current increase from an elevated voltage bias, the current-voltage (I-V) curves display strong negative differential resistance (NDR) and perfect current-switching characteristics. The asymmetric DNA chain differs in mechanical stability under inverse voltages and the I-V curve is asymmetric about inverse biases, which can be used to understand recent transport experiments on DNA chains, and meanwhile provides a new strategy to realize NDR in molecular junctions and other low-dimensional quantum systems.

摘要

电流诱导力可以激发分子、聚合物和其他低维材料,进而通过霍尔斯坦相互作用产生有效的栅极电压。在此,以短的不对称DNA结为例,并采用朗之万方法,我们发现当有效栅极电压对电荷传输的抑制超过因电压偏置升高而导致的电流增加时,电流-电压(I-V)曲线呈现出强烈的负微分电阻(NDR)和完美的电流开关特性。不对称DNA链在反向电压下的机械稳定性不同,且I-V曲线关于反向偏置不对称,这可用于理解近期关于DNA链的输运实验,同时为在分子结和其他低维量子系统中实现负微分电阻提供了一种新策略。

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