Quarati F G A, Dorenbos P, Mougeot X
AP, RST, FAME, Delft University of Technology, Mekelweg 15, 2629JB Delft, The Netherlands; Gonitec BV, Johannes Bildersstraat 60, 2596EJ Den Haag, The Netherlands.
AP, RST, FAME, Delft University of Technology, Mekelweg 15, 2629JB Delft, The Netherlands.
Appl Radiat Isot. 2016 Feb;108:30-34. doi: 10.1016/j.apradiso.2015.11.080. Epub 2015 Dec 11.
We measured with unprecedented accuracy key features of the (138)La radioactive decays as β particle energy distribution from 0.5 keV to the end-point and ratios of electron capture probabilities PL/PK, PM/PK and PM/PL. This was achieved by making use of LaBr3:Ce and CeBr3 scintillator detectors. The advantage of the presented technique relies on the double role of LaBr3:Ce as source of (138)La and detector medium resulting in a relatively efficient counting statistics and unaltered β energy detection. The experimental results are compared to advanced computational techniques and significant deviation is found below 20 keV with the computational spectrum showing a 5% excess of β particle relative to the experimental spectrum at 10 keV.
我们以前所未有的精度测量了¹³⁸La放射性衰变的关键特征,如从0.5 keV到端点的β粒子能量分布以及电子俘获概率比PL/PK、PM/PK和PM/PL。这是通过使用LaBr₃:Ce和CeBr₃闪烁体探测器实现的。所提出技术的优势在于LaBr₃:Ce作为¹³⁸La源和探测器介质的双重作用,从而产生相对高效的计数统计和未改变的β能量探测。将实验结果与先进的计算技术进行了比较,发现在20 keV以下存在显著偏差,计算谱在10 keV处显示出比实验谱多5%的β粒子。