Pascarelli S, Mathon O, Mairs T, Kantor I, Agostini G, Strohm C, Pasternak S, Perrin F, Berruyer G, Chappelet P, Clavel C, Dominguez M C
European Synchrotron Radiation Facility, 71 Avenue des Martyrs, 38000 Grenoble, France.
J Synchrotron Radiat. 2016 Jan;23(1):353-68. doi: 10.1107/S160057751501783X. Epub 2016 Jan 1.
The European Synchrotron Radiation Facility has recently made available to the user community a facility totally dedicated to Time-resolved and Extreme-conditions X-ray Absorption Spectroscopy--TEXAS. Based on an upgrade of the former energy-dispersive XAS beamline ID24, it provides a unique experimental tool combining unprecedented brilliance (up to 10(14) photons s(-1) on a 4 µm × 4 µm FWHM spot) and detection speed for a full EXAFS spectrum (100 ps per spectrum). The science mission includes studies of processes down to the nanosecond timescale, and investigations of matter at extreme pressure (500 GPa), temperature (10000 K) and magnetic field (30 T). The core activities of the beamline are centered on new experiments dedicated to the investigation of extreme states of matter that can be maintained only for very short periods of time. Here the infrastructure, optical scheme, detection systems and sample environments used to enable the mission-critical performance are described, and examples of first results on the investigation of the electronic and local structure in melts at pressure and temperature conditions relevant to the Earth's interior and in laser-shocked matter are given.
欧洲同步辐射装置最近向用户群体提供了一个完全致力于时间分辨和极端条件下X射线吸收光谱学的设施——TEXAS。它基于对 former 能量色散X射线吸收光谱线ID24的升级,提供了一种独特的实验工具,结合了前所未有的亮度(在4 µm×4 µm 半高宽光斑上高达10¹⁴ 光子·秒⁻¹)和全扩展X射线吸收精细结构光谱的检测速度(每光谱100皮秒)。科学任务包括对纳秒时间尺度以下过程的研究,以及对极端压力(500 GPa)、温度(10000 K)和磁场(30 T)下物质的研究。该光束线的核心活动集中在致力于研究只能在极短时间内维持的物质极端状态的新实验上。这里描述了用于实现关键任务性能的基础设施、光学方案、检测系统和样品环境,并给出了在与地球内部相关的压力和温度条件下以及激光冲击物质中对熔体的电子和局部结构进行研究的首批结果示例。