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一维两步外延生长中的普遍性与标度律

Universality and scaling in two-step epitaxial growth in one dimension.

作者信息

Tokar V I, Dreyssé H

机构信息

IPCMS, Université de Strasbourg-CNRS, UMR 7504, 23 rue du Loess, F-67034 Strasbourg, France.

出版信息

Phys Rev E Stat Nonlin Soft Matter Phys. 2015 Dec;92(6):062407. doi: 10.1103/PhysRevE.92.062407. Epub 2015 Dec 28.

Abstract

Irreversible one-dimensional (1D) epitaxial growth at small coverages via the recently suggested two-step growth protocol [Tokar and Dreyssé, Surf. Sci. 637-638, 116 (2015)] has been studied with the use of the kinetic Monte Carlo and the rate-equation techniques. It has been found that similar to the two-dimensional (2D) case the island capture zones could be accurately approximated with the Gamma probability distribution (GD). Coverage independence of the average island sizes grown at the first step that was also found in two dimensions was observed. In contrast to 2D case, the shape parameter of the GD was also found to be coverage-independent. Using these two constants as the input, an analytical approach that allowed for the description of the commonly studied statistical distributions to the accuracy of about 2% has been developed. Furthermore, it was established that the distributions of the island sizes and the interisland gaps grown via the two-step protocol were about 50% narrower than in the case of nucleation on random defects, which can be of practical importance. Equivalence between the GD shape of the island size distribution in the scaling regime and the linear dependence of the capture numbers on the island size in the rate-equation approach has been proved.

摘要

通过最近提出的两步生长协议[托卡尔和德雷塞,《表面科学》637 - 638卷,116页(2015年)],在小覆盖率下的不可逆一维(1D)外延生长已通过动力学蒙特卡罗和速率方程技术进行了研究。结果发现,与二维(2D)情况类似,岛捕获区可以用伽马概率分布(GD)精确近似。观察到在第一步生长的平均岛尺寸与覆盖率无关,这在二维情况下也已发现。与二维情况不同的是,还发现GD的形状参数也与覆盖率无关。以这两个常数作为输入,已开发出一种解析方法,该方法能够将常见研究的统计分布描述到约2%的精度。此外,已确定通过两步协议生长的岛尺寸和岛间间隙的分布比在随机缺陷上成核的情况窄约50%,这可能具有实际重要性。已证明在标度 regime 中岛尺寸分布的GD形状与速率方程方法中捕获数对岛尺寸的线性依赖性之间的等效性。

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