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掺杂诱导的 d(4)莫特绝缘体中的铁磁性和可能的三重态配对。

Doping-Induced Ferromagnetism and Possible Triplet Pairing in d(4) Mott Insulators.

机构信息

Central European Institute of Technology, Masaryk University, Kotlářská 2, 61137 Brno, Czech Republic.

Max Planck Institute for Solid State Research, Heisenbergstrasse 1, D-70569 Stuttgart, Germany.

出版信息

Phys Rev Lett. 2016 Jan 8;116(1):017203. doi: 10.1103/PhysRevLett.116.017203.

Abstract

We study the effects of electron doping in Mott insulators containing d(4) ions such as Ru(4+), Os(4+), Rh(5+), and Ir(5+) with J=0 singlet ground state. Depending on the strength of the spin-orbit coupling, the undoped systems are either nonmagnetic or host an unusual, excitonic magnetism arising from a condensation of the excited J=1 triplet states of t(2g)(4). We find that the interaction between J excitons and doped carriers strongly supports ferromagnetism, converting both the nonmagnetic and antiferromagnetic phases of the parent insulator into a ferromagnetic metal, and further to a nonmagnetic metal. Close to the ferromagnetic phase, the low-energy spin response is dominated by intense paramagnon excitations that may act as mediators of a triplet pairing.

摘要

我们研究了具有 J=0 单线基态的 d(4)离子(如 Ru(4+)、Os(4+)、Rh(5+)和 Ir(5+))的莫特绝缘体中电子掺杂的影响。根据自旋轨道耦合的强度,未掺杂的系统要么是非磁性的,要么存在一种不寻常的激子磁性,这种磁性源于 t(2g)(4)的激发 J=1 三重态的凝聚。我们发现 J 激子与掺杂载流子之间的相互作用强烈支持铁磁性,将母体绝缘体的非磁性和反铁磁相都转化为铁磁金属,进一步转化为非磁金属。在铁磁相附近,低能自旋响应主要由强烈的 paramagnon 激发主导,这些激发可能作为三重态配对的介导者。

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